Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives
Тип публикации: Journal Article
Дата публикации: 2017-08-18
scimago Q1
Tоп 10% SciMago
wos Q1
white level БС1
SJR: 1.352
CiteScore: 9
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Краткое описание
Photoinduced metal-free atom transfer radical polymerization (ATRP) activated by highly conjugated electron-rich thienothiophene derivatives, namely 4-[2-(4-diphenylaminophenyl)-thieno[3,2-b]thiophen-3-yl]benzonitrile (TT-TPA), 4-[2,5-bis(4-diphenylaminophenyl)-thieno[3,2-b]thiophen-3-yl]benzonitrile (TPA-TT-TPA), 4-(2-(4-(1,2,2-triphenylvinyl)phenyl) thieno[3,2-b]thiophen-3-yl)benzonitrile (TT-TPE) and 4-(2,5-bis(4-(1,2,2-triphenylvinyl)phenyl)thieno[3,2-b]thiophen-3- yl)benzonitrile (TPE-TT-TPE) is reported. Polymerization of methyl methacrylate (MMA) is efficiently activated and deactivated with light, forming polymers with controlled the molecular weight characteristics, dispersity, and chain end functionality. Polymerization studies and DFT calculations revealed that TT-TPA is the most efficient activator due to the favorable thermodynamic properties.
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Kutahya C. et al. Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives // Macromolecules. 2017. Vol. 50. No. 17. pp. 6903-6910.
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Kutahya C., Allushi A., Isci R., Kreutzer J., Öztürk T., Yilmaz G., Yagci Y. Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives // Macromolecules. 2017. Vol. 50. No. 17. pp. 6903-6910.
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TY - JOUR
DO - 10.1021/acs.macromol.7b01335
UR - https://doi.org/10.1021/acs.macromol.7b01335
TI - Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives
T2 - Macromolecules
AU - Kutahya, Ceren
AU - Allushi, Andrit
AU - Isci, Recep
AU - Kreutzer, Johannes
AU - Öztürk, Turan
AU - Yilmaz, Gorkem
AU - Yagci, Yusuf
PY - 2017
DA - 2017/08/18
PB - American Chemical Society (ACS)
SP - 6903-6910
IS - 17
VL - 50
SN - 0024-9297
SN - 1520-5835
ER -
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@article{2017_Kutahya,
author = {Ceren Kutahya and Andrit Allushi and Recep Isci and Johannes Kreutzer and Turan Öztürk and Gorkem Yilmaz and Yusuf Yagci},
title = {Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives},
journal = {Macromolecules},
year = {2017},
volume = {50},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.macromol.7b01335},
number = {17},
pages = {6903--6910},
doi = {10.1021/acs.macromol.7b01335}
}
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MLA
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Kutahya, Ceren, et al. “Photoinduced Metal-Free Atom Transfer Radical Polymerization Using Highly Conjugated Thienothiophene Derivatives.” Macromolecules, vol. 50, no. 17, Aug. 2017, pp. 6903-6910. https://doi.org/10.1021/acs.macromol.7b01335.
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