volume 22 issue 2 pages 673-679

Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy

Publication typeJournal Article
Publication date2022-01-10
scimago Q1
wos Q1
SJR2.967
CiteScore14.9
Impact factor9.1
ISSN15306984, 15306992
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
Free-standing few-layered MoSe2 nanosheet stacks optoelectronic signatures are analyzed by using light compatible in situ transmission electron microscopy (TEM) utilizing an optical TEM holder allowing for the simultaneous mechanical deformation, electrical probing and light illumination of a sample. Two types of deformation, namely, (i) bending of nanosheets perpendicular to their basal atomic planes and (ii) edge deformation parallel to the basal atomic planes, lead to two distinctly different optomechanical performances of the nanosheet stacks. The former deformation induces a stable but rather marginal increase in photocurrent, whereas the latter mode is prone to unstable nonsystematic photocurrent value changes and a red-shifted photocurrent spectrum. The experimental results are verified by ab initio calculations using density functional theory (DFT).
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GOST |
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GOST Copy
Zhang C. et al. Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy // Nano Letters. 2022. Vol. 22. No. 2. pp. 673-679.
GOST all authors (up to 50) Copy
Zhang C., Larionov K. V., Firestein K. L., Fernando J. F. S., Lewis C. E., Sorokin P. B., Golberg D. Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy // Nano Letters. 2022. Vol. 22. No. 2. pp. 673-679.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.nanolett.1c03796
UR - https://doi.org/10.1021/acs.nanolett.1c03796
TI - Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy
T2 - Nano Letters
AU - Zhang, Chao
AU - Larionov, Konstantin V.
AU - Firestein, Konstantin L
AU - Fernando, Joseph F S
AU - Lewis, Courtney Elyce
AU - Sorokin, Pavel B.
AU - Golberg, Dmitri
PY - 2022
DA - 2022/01/10
PB - American Chemical Society (ACS)
SP - 673-679
IS - 2
VL - 22
PMID - 35007088
SN - 1530-6984
SN - 1530-6992
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2022_Zhang,
author = {Chao Zhang and Konstantin V. Larionov and Konstantin L Firestein and Joseph F S Fernando and Courtney Elyce Lewis and Pavel B. Sorokin and Dmitri Golberg},
title = {Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy},
journal = {Nano Letters},
year = {2022},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.nanolett.1c03796},
number = {2},
pages = {673--679},
doi = {10.1021/acs.nanolett.1c03796}
}
MLA
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MLA Copy
Zhang, Chao, et al. “Optomechanical Properties of MoSe2Nanosheets as Revealed by in Situ Transmission Electron Microscopy.” Nano Letters, vol. 22, no. 2, Jan. 2022, pp. 673-679. https://doi.org/10.1021/acs.nanolett.1c03796.