Organometallics

, том 34 , издание 14 , страницы 3559-3570

Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBuⁱ2 (X = H, Cl, Buⁱ), Catalyzed by Zr η⁵ Complexes

Тип публикации: Journal Article

Дата публикации: 2015-07-08

American Chemical Society (ACS)

Organometallics

SCImago Q2

WOS Q2

БС1

SJR: 0.55

CiteScore: 4.6

Impact factor: 2.4

ISSN: 02767333, 15206041

DOI: 10.1021/acs.organomet.5b00370

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Organic Chemistry

Inorganic Chemistry

Physical and Theoretical Chemistry

Краткое описание

The zirconocene complexes L2ZrCl2 (L = C5H5, C5H4Me, Ind, C5Me5; L2 = rac-Me2C(2-Me-4-But-C5H2)2, meso-Me2C(2-Me-4-But-C5H2)2, rac-Me2C(3-But-C5H3)2, rac-Me2C(Ind)2, rac-Me2Si(Ind)2, and rac-C2H4(Ind)2) were tested as catalysts in alkene hydroalumination by the isobutylalanes XAlBui2 (X = H, Cl, Bui). A low-temperature NMR spectroscopy study on the structure and dynamics of Zr,Al intermediates formed in the L2ZrCl2–XAlBui2 systems showed that the intra- and intermolecular exchange in the bimetallic clusters, controlled by the steric factor of the η5 ligand and organoaluminum compound nature, determines the activity of the whole catalytic system.

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Parfenova L. V. et al. Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBui2 (X = H, Cl, Bui), Catalyzed by Zr η5 Complexes // Organometallics. 2015. Vol. 34. No. 14. pp. 3559-3570.

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Parfenova L. V., Kovyazin P. V., Nifant'ev I. E., Khalilov L. M., Dzhemilev U. M. Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBui2 (X = H, Cl, Bui), Catalyzed by Zr η5 Complexes // Organometallics. 2015. Vol. 34. No. 14. pp. 3559-3570.

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TY - JOUR

DO - 10.1021/acs.organomet.5b00370

UR - https://pubs.acs.org/doi/10.1021/acs.organomet.5b00370

TI - Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBui2 (X = H, Cl, Bui), Catalyzed by Zr η5 Complexes

T2 - Organometallics

AU - Parfenova, Lyudmila V.

AU - Kovyazin, Pavel V

AU - Nifant'ev, Ilya E.

AU - Khalilov, Leonard M.

AU - Dzhemilev, Usein M

PY - 2015

DA - 2015/07/08

PB - American Chemical Society (ACS)

SP - 3559-3570

IS - 14

VL - 34

SN - 0276-7333

SN - 1520-6041

ER -

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@article{2015_Parfenova,

author = {Lyudmila V. Parfenova and Pavel V Kovyazin and Ilya E. Nifant'ev and Leonard M. Khalilov and Usein M Dzhemilev},

title = {Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBui2 (X = H, Cl, Bui), Catalyzed by Zr η5 Complexes},

journal = {Organometallics},

year = {2015},

volume = {34},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://pubs.acs.org/doi/10.1021/acs.organomet.5b00370},

number = {14},

pages = {3559--3570},

doi = {10.1021/acs.organomet.5b00370}

}

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Parfenova, Lyudmila V., et al. “Role of Zr,Al Hydride Intermediate Structure and Dynamics in Alkene Hydroalumination with XAlBui2 (X = H, Cl, Bui), Catalyzed by Zr η5 Complexes.” Organometallics, vol. 34, no. 14, Jul. 2015, pp. 3559-3570. https://pubs.acs.org/doi/10.1021/acs.organomet.5b00370.

Издатель

American Chemical Society (ACS)

Журнал

Organometallics

SCImago Q2

WOS Q2

БС1

SJR

0.55

CiteScore

4.6

Impact factor