Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives
Publication type: Journal Article
Publication date: 2020-06-17
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
32610921
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
A visible-light-mediated decarboxylative tandem carbocyclization of acrylamide-tethered alkylidenecyclopropanes with phenyliodine(III) diacetate and various aliphatic acids has been reported in this paper. An alkyl radical in situ generated from phenyliodine(III) dicarboxylates upon visible-light irradiation catalyzed by fac-Ir(ppy)3 adds to the less hindered central carbon of alkylidenecyclopropane to initiate the tandem annulation, generating tetracyclic benzazepine derivatives in moderate to good yields with broad substrate scope under mild conditions.
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21
Total citations:
21
Citations from 2024:
12
(57%)
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GOST
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Zhang X. et al. Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives // Organic Letters. 2020. Vol. 22. No. 13. pp. 5212-5216.
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Zhang X., Ning C., Long Y. J., Wei Yin 尹., Shi M. Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives // Organic Letters. 2020. Vol. 22. No. 13. pp. 5212-5216.
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RIS
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TY - JOUR
DO - 10.1021/acs.orglett.0c01856
UR - https://doi.org/10.1021/acs.orglett.0c01856
TI - Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives
T2 - Organic Letters
AU - Zhang, Xiao-Yu
AU - Ning, Chao
AU - Long, Yong Jie
AU - Wei Yin, 尹维
AU - Shi, Min
PY - 2020
DA - 2020/06/17
PB - American Chemical Society (ACS)
SP - 5212-5216
IS - 13
VL - 22
PMID - 32610921
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
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@article{2020_Zhang,
author = {Xiao-Yu Zhang and Chao Ning and Yong Jie Long and 尹维 Wei Yin and Min Shi},
title = {Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives},
journal = {Organic Letters},
year = {2020},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acs.orglett.0c01856},
number = {13},
pages = {5212--5216},
doi = {10.1021/acs.orglett.0c01856}
}
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MLA
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Zhang, Xiao-Yu, et al. “Visible-Light-Mediated Decarboxylative Tandem Carbocyclization of Acrylamide-Attached Alkylidenecyclopropanes: Access to Polycyclic Benzazepine Derivatives.” Organic Letters, vol. 22, no. 13, Jun. 2020, pp. 5212-5216. https://doi.org/10.1021/acs.orglett.0c01856.