Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity
2
GoldenKeys High-tech Materials Co., Ltd., Building B, Innovation & Entrepreneurship Park, Guian New Area, Guian 550025, Guizhou Province, China
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Publication type: Journal Article
Publication date: 2020-08-04
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
32806188
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
The use of arene/Ru/TsDPEN catalysts bearing a heterocyclic group on the TsDPEN in the asymmetric transfer hydrogenation (ATH) of dihydroisoquinolines (DHIQs) containing meta- or para-substituted aromatic groups at the 1-position results in the formation of products of high enantiomeric excess. Previously, only 1-(ortho-substituted)aryl DHIQs, or with an electron-rich fused ring gave products with high enantioselectivity; therefore, this approach solves a long-standing challenge for imine ATH.
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27
Total citations:
27
Citations from 2024:
12
(44.44%)
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GOST
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Barrios Rivera J., Xu Y., Wills M. R. Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity // Organic Letters. 2020. Vol. 22. No. 16. pp. 6283-6287.
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Barrios Rivera J., Xu Y., Wills M. R. Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity // Organic Letters. 2020. Vol. 22. No. 16. pp. 6283-6287.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.orglett.0c02034
UR - https://doi.org/10.1021/acs.orglett.0c02034
TI - Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity
T2 - Organic Letters
AU - Barrios Rivera, Jonathan
AU - Xu, Yingjian
AU - Wills, M. R.
PY - 2020
DA - 2020/08/04
PB - American Chemical Society (ACS)
SP - 6283-6287
IS - 16
VL - 22
PMID - 32806188
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Barrios Rivera,
author = {Jonathan Barrios Rivera and Yingjian Xu and M. R. Wills},
title = {Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity},
journal = {Organic Letters},
year = {2020},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.orglett.0c02034},
number = {16},
pages = {6283--6287},
doi = {10.1021/acs.orglett.0c02034}
}
Cite this
MLA
Copy
Barrios Rivera, Jonathan, et al. “Asymmetric Transfer Hydrogenation of Unhindered and Non-Electron-Rich 1-Aryl Dihydroisoquinolines with High Enantioselectivity.” Organic Letters, vol. 22, no. 16, Aug. 2020, pp. 6283-6287. https://doi.org/10.1021/acs.orglett.0c02034.