Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes
Zi Lu Wang
1
,
Ying Wang
1
,
Jian Lin Xu
1
,
Meng Zhao
1
,
Kai Yang Dai
1
,
Cui Cui Shan
1
,
Yunhe Xu
1, 2
Publication type: Journal Article
Publication date: 2021-06-07
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
34096735
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
Unprecedented copper-catalyzed regiodivergent hydrosilylation reactions of substituted 1,3-dienes with hydrosilanes have been developed. The 1,2- and 1,4-hydrosilylations of 1-(hetero)aryl-substituted 1,3-dienes were highly selectively controlled via variation of the catalytic systems. Meanwhile, the 1,4-hydrosilylation reaction of 2-aryl-substituted 1,3-dienes with diphenylsilane was also successfully realized for the first time. These methods provide convenient and efficient approaches for the synthesis of structurally diverse allylsilanes.
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42
Total citations:
42
Citations from 2024:
18
(42.86%)
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GOST
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Wang Z. L. et al. Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes // Organic Letters. 2021. Vol. 23. No. 12. pp. 4736-4742.
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Wang Z. L., Wang Y., Xu J. L., Zhao M., Dai K. Y., Shan C. C., Xu Y. Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes // Organic Letters. 2021. Vol. 23. No. 12. pp. 4736-4742.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.orglett.1c01455
UR - https://doi.org/10.1021/acs.orglett.1c01455
TI - Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes
T2 - Organic Letters
AU - Wang, Zi Lu
AU - Wang, Ying
AU - Xu, Jian Lin
AU - Zhao, Meng
AU - Dai, Kai Yang
AU - Shan, Cui Cui
AU - Xu, Yunhe
PY - 2021
DA - 2021/06/07
PB - American Chemical Society (ACS)
SP - 4736-4742
IS - 12
VL - 23
PMID - 34096735
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Wang,
author = {Zi Lu Wang and Ying Wang and Jian Lin Xu and Meng Zhao and Kai Yang Dai and Cui Cui Shan and Yunhe Xu},
title = {Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes},
journal = {Organic Letters},
year = {2021},
volume = {23},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acs.orglett.1c01455},
number = {12},
pages = {4736--4742},
doi = {10.1021/acs.orglett.1c01455}
}
Cite this
MLA
Copy
Wang, Zi Lu, et al. “Synthesis of Structurally Diverse Allylsilanes via Copper-Catalyzed Regiodivergent Hydrosilylation of 1,3-Dienes.” Organic Letters, vol. 23, no. 12, Jun. 2021, pp. 4736-4742. https://doi.org/10.1021/acs.orglett.1c01455.