Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide
Publication type: Journal Article
Publication date: 2022-03-17
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
35297636
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
Thiolation of carboxylic acids using a disulfide reagent having tetrafluoropyridinyl groups is described. The light-mediated process is performed using an acridine-type photocatalyst. Primary, secondary, tertiary, and heteroatom-substituted carboxylic acids can be thiolated, and the method can be applied to the late-stage modification of a range of naturally occurring compounds and drugs. The fluorinated pyridine fragment is believed to enable the C-S bond formation. The resulting sulfides were used as redox-active radical precursors.
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45
Total citations:
45
Citations from 2024:
28
(62%)
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GOST
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Zubkov M. O. et al. Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide // Organic Letters. 2022. Vol. 24. No. 12. pp. 2354-2358.
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Zubkov M. O., Kosobokov M. D., Levin V. V., Dilman A. D. Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide // Organic Letters. 2022. Vol. 24. No. 12. pp. 2354-2358.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.orglett.2c00549
UR - https://doi.org/10.1021/acs.orglett.2c00549
TI - Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide
T2 - Organic Letters
AU - Zubkov, Mikhail O
AU - Kosobokov, Mikhail D
AU - Levin, Vitalij V
AU - Dilman, Alexander D
PY - 2022
DA - 2022/03/17
PB - American Chemical Society (ACS)
SP - 2354-2358
IS - 12
VL - 24
PMID - 35297636
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2022_Zubkov,
author = {Mikhail O Zubkov and Mikhail D Kosobokov and Vitalij V Levin and Alexander D Dilman},
title = {Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide},
journal = {Organic Letters},
year = {2022},
volume = {24},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acs.orglett.2c00549},
number = {12},
pages = {2354--2358},
doi = {10.1021/acs.orglett.2c00549}
}
Cite this
MLA
Copy
Zubkov, Mikhail O., et al. “Photocatalyzed Decarboxylative Thiolation of Carboxylic Acids Enabled by Fluorinated Disulfide.” Organic Letters, vol. 24, no. 12, Mar. 2022, pp. 2354-2358. https://doi.org/10.1021/acs.orglett.2c00549.