Organic Letters

, том 19 , издание 19 , страницы 5204-5207

(Z)-Selective Hydrosilylation of Terminal Alkynes with HSiMe(OSiMe₃)₂ Catalyzed by a Ruthenium Complex Containing an N-Heterocyclic Carbene

Тип публикации: Journal Article

Дата публикации: 2017-09-08

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Organic Letters

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SJR: 1.007

CiteScore: 8.7

Impact factor: 5

ISSN: 15237060, 15237052

DOI: 10.1021/acs.orglett.7b02477

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PubMed ID: 28885855

Organic Chemistry

Biochemistry

Physical and Theoretical Chemistry

Краткое описание

The N-heterocyclic-carbene-ligated ruthenium complex [RuHCl(CO)(H2IMes)(PCy3)] exhibits high catalytic activity for the (Z)-selective hydrosilylation of various terminal alkynes with 1,1,1,3,5,5,5-heptamethyltrisiloxane (HSiMe(OSiMe3)2). The stereoretentive derivatization of the (Z)-alkenylsiloxanes allows the synthesis of biologically active compounds, e.g. potent antitumor agents and inhibitors for induced-NO synthase.

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Mutoh Y., Mohara Y., SAITO S. (Z)-Selective Hydrosilylation of Terminal Alkynes with HSiMe(OSiMe3)2 Catalyzed by a Ruthenium Complex Containing an N-Heterocyclic Carbene // Organic Letters. 2017. Vol. 19. No. 19. pp. 5204-5207.

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TY - JOUR

DO - 10.1021/acs.orglett.7b02477

UR - https://doi.org/10.1021/acs.orglett.7b02477

TI - (Z)-Selective Hydrosilylation of Terminal Alkynes with HSiMe(OSiMe3)2 Catalyzed by a Ruthenium Complex Containing an N-Heterocyclic Carbene

T2 - Organic Letters

AU - Mutoh, Yuichiro

AU - Mohara, Yusei

AU - SAITO, Shinichi

PY - 2017

DA - 2017/09/08

PB - American Chemical Society (ACS)

SP - 5204-5207

IS - 19

VL - 19

PMID - 28885855

SN - 1523-7060

SN - 1523-7052

ER -

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@article{2017_Mutoh,

author = {Yuichiro Mutoh and Yusei Mohara and Shinichi SAITO},

title = {(Z)-Selective Hydrosilylation of Terminal Alkynes with HSiMe(OSiMe3)2 Catalyzed by a Ruthenium Complex Containing an N-Heterocyclic Carbene},

journal = {Organic Letters},

year = {2017},

volume = {19},

publisher = {American Chemical Society (ACS)},

month = {sep},

url = {https://doi.org/10.1021/acs.orglett.7b02477},

number = {19},

pages = {5204--5207},

doi = {10.1021/acs.orglett.7b02477}

}

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Mutoh, Yuichiro, et al. “(Z)-Selective Hydrosilylation of Terminal Alkynes with HSiMe(OSiMe3)2 Catalyzed by a Ruthenium Complex Containing an N-Heterocyclic Carbene.” Organic Letters, vol. 19, no. 19, Sep. 2017, pp. 5204-5207. https://doi.org/10.1021/acs.orglett.7b02477.

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American Chemical Society (ACS)

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Organic Letters

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