Organic Letters

, том 20 , издание 15 , страницы 4632-4636

Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles

Тип публикации: Journal Article

Дата публикации: 2018-07-26

American Chemical Society (ACS)

Organic Letters

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SJR: 1.235

CiteScore: 8.7

Impact factor: 5

ISSN: 15237060, 15237052

DOI: 10.1021/acs.orglett.8b01910

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PubMed ID: 30047738

Organic Chemistry

Biochemistry

Physical and Theoretical Chemistry

Краткое описание

The rhodium(III)-catalyzed cross-coupling of (hetero)aryl nitrones with Morita-Baylis-Hillman (MBH) adducts is described. An allylated intermediate derived from aryl nitrones and MBH adducts allows the formation of bridged cyclic compounds via an exotype [3 + 2] cycloaddition. In sharp contrast, electron-rich indolinyl or aniline substrates were found to couple with MBH adducts to generate naphthalene or carbazole derivatives, respectively.

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Organic Letters	Organic Letters, 6, 15% Organic Letters 6 публикаций, 15%
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Pandey A. K. et al. Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles // Organic Letters. 2018. Vol. 20. No. 15. pp. 4632-4636.

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Pandey A. K., KANG D., Han S. H., Lee H. Y., Mishra N. K., Kim H. S., Jung Y., Hong S., Kim I. S. Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles // Organic Letters. 2018. Vol. 20. No. 15. pp. 4632-4636.

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TY - JOUR

DO - 10.1021/acs.orglett.8b01910

UR - https://doi.org/10.1021/acs.orglett.8b01910

TI - Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles

T2 - Organic Letters

AU - Pandey, Ashok Kumar

AU - KANG, DA-HYE

AU - Han, Sang Hoon

AU - Lee, Hee Young

AU - Mishra, Neeraj Kumar

AU - Kim, H S

AU - Jung, Young-Hoon

AU - Hong, Sungwoo

AU - Kim, In Su

PY - 2018

DA - 2018/07/26

PB - American Chemical Society (ACS)

SP - 4632-4636

IS - 15

VL - 20

PMID - 30047738

SN - 1523-7060

SN - 1523-7052

ER -

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@article{2018_Pandey,

author = {Ashok Kumar Pandey and DA-HYE KANG and Sang Hoon Han and Hee Young Lee and Neeraj Kumar Mishra and H S Kim and Young-Hoon Jung and Sungwoo Hong and In Su Kim},

title = {Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles},

journal = {Organic Letters},

year = {2018},

volume = {20},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://doi.org/10.1021/acs.orglett.8b01910},

number = {15},

pages = {4632--4636},

doi = {10.1021/acs.orglett.8b01910}

}

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Pandey, Ashok Kumar, et al. “Reactivity of Morita–Baylis–Hillman Adducts in C–H Functionalization of (Hetero)aryl Nitrones: Access to Bridged Cycles and Carbazoles.” Organic Letters, vol. 20, no. 15, Jul. 2018, pp. 4632-4636. https://doi.org/10.1021/acs.orglett.8b01910.