Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids.
Publication type: Journal Article
Publication date: 2018-12-07
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
30525672
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
We developed a ruthenium-catalyzed reductive ester synthesis from aldehydes or ketones and carboxylic acids using carbon monoxide as a deoxygenative agent. Multiple factors influencing the outcome of the reaction were investigated. Best results were obtained for commercially available and inexpensive benzene ruthenium chloride; as low as 0.5 mol % of the catalyst is sufficient for efficient reaction. Competitive studies demonstrated that the presence of even 1000 equiv of alcohol in the reaction mixture does not lead to the corresponding ester, which clearly indicates that the process is not a simple reductive esterification but a novel type of Ru-catalyzed redox process.
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13
Total citations:
13
Citations from 2024:
2
(15.38%)
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GOST
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Runikhina S. A. et al. Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids. // Organic Letters. 2018. Vol. 20. No. 24. pp. 7856-7859.
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Runikhina S. A., Usanov D. A., Chizhov A. O., Chusov D. Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids. // Organic Letters. 2018. Vol. 20. No. 24. pp. 7856-7859.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.orglett.8b03375
UR - https://doi.org/10.1021/acs.orglett.8b03375
TI - Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids.
T2 - Organic Letters
AU - Runikhina, Sofiya A
AU - Usanov, Dmitry A.
AU - Chizhov, A. O.
AU - Chusov, Denis
PY - 2018
DA - 2018/12/07
PB - American Chemical Society (ACS)
SP - 7856-7859
IS - 24
VL - 20
PMID - 30525672
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Runikhina,
author = {Sofiya A Runikhina and Dmitry A. Usanov and A. O. Chizhov and Denis Chusov},
title = {Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids.},
journal = {Organic Letters},
year = {2018},
volume = {20},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.orglett.8b03375},
number = {24},
pages = {7856--7859},
doi = {10.1021/acs.orglett.8b03375}
}
Cite this
MLA
Copy
Runikhina, Sofiya A., et al. “Atom- and Step-Economical Ruthenium-Catalyzed Synthesis of Esters from Aldehydes or Ketones and Carboxylic Acids..” Organic Letters, vol. 20, no. 24, Dec. 2018, pp. 7856-7859. https://doi.org/10.1021/acs.orglett.8b03375.
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