volume 21 issue 20 pages 8373-8377

Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides

Publication typeJournal Article
Publication date2019-10-01
scimago Q1
wos Q1
SJR1.235
CiteScore8.7
Impact factor5.0
ISSN15237060, 15237052
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
An enantioselective borylative cyclization cascade utilizing cyclic imides has been developed. We employ a highly enantioselective borylcupration process that includes a 1,2-addition to a cyclic imide. The products contain a valuable hemiaminal and boronate handle for further elaborations within a congested framework. This work demonstrates the utility of cyclic imides as simple precursors to unlock access to sought-after polycyclic indolines. Futhermore, this report highlights the capability to harness reactive catalytic intermediates to exploit otherwise unreactive functional groups.
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Whyte A. F. et al. Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides // Organic Letters. 2019. Vol. 21. No. 20. pp. 8373-8377.
GOST all authors (up to 50) Copy
Whyte A. F., Torelli A., Mirabi B., Lautens M. Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides // Organic Letters. 2019. Vol. 21. No. 20. pp. 8373-8377.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.orglett.9b03144
UR - https://doi.org/10.1021/acs.orglett.9b03144
TI - Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides
T2 - Organic Letters
AU - Whyte, Andrew F.
AU - Torelli, Alexa
AU - Mirabi, Bijan
AU - Lautens, Mark
PY - 2019
DA - 2019/10/01
PB - American Chemical Society (ACS)
SP - 8373-8377
IS - 20
VL - 21
PMID - 31573212
SN - 1523-7060
SN - 1523-7052
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2019_Whyte,
author = {Andrew F. Whyte and Alexa Torelli and Bijan Mirabi and Mark Lautens},
title = {Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides},
journal = {Organic Letters},
year = {2019},
volume = {21},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.orglett.9b03144},
number = {20},
pages = {8373--8377},
doi = {10.1021/acs.orglett.9b03144}
}
MLA
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MLA Copy
Whyte, Andrew F., et al. “Enantioselective Copper-Catalyzed Borylative Cyclization with Cyclic Imides.” Organic Letters, vol. 21, no. 20, Oct. 2019, pp. 8373-8377. https://doi.org/10.1021/acs.orglett.9b03144.