New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals
Alexey S Berezin
1
,
Irina Yu. Bagryanskaya
2
,
Valery K. Brel
3
,
Xiuze Hei
4
,
Oleg I. Artyushin
3
,
Lev E Zelenkov
5
,
Ivan I Shishkin
5
,
Jing Li
4
Тип публикации: Journal Article
Дата публикации: 2022-06-27
scimago Q1
wos Q1
БС1
SJR: 1.921
CiteScore: 14.5
Impact factor: 8.2
ISSN: 19448244, 19448252
PubMed ID:
35758694
General Materials Science
Краткое описание
Inorganic-organic hybrid luminescent materials have received great attention for their potential applications in a wide range of clean/renewable energy-related areas, including photovoltaics and solid-state lighting. Herein, we present a unique and general "Mn + Cu" approach by blending two earth-abundant luminogenic metals, manganese and copper, within a single ionic structure to construct a remarkable family of low-cost and multifunctional hybrid materials featuring dual emission, as well as triboluminescence and second-harmonic generation response. The novel hybrid materials are made of diphosphine dioxide-chelated [Mn(O∧O)3]2+ cations and various anionic [CuxIy](y-x)- clusters, ensuring manifestation of dual phosphorescence streamed from octahedral Mn2+ ions (605-648 nm) and iodocuprate anions (480-728 nm). Noteworthily, the relative ratio of the emission bands, and hence a resulting emission chromaticity, can be tuned in a wide range through modification of cluster [CuxIy](y-x)- modules. The structural diversity, enhanced robustness, and up to 100% luminescence quantum yield make the designed materials promising phosphors for lighting and sensing applications.
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ГОСТ
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Artem'ev A. V. et al. New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals // ACS applied materials & interfaces. 2022. Vol. 14. No. 27. pp. 31000-31009.
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Artem'ev A. V., Davydova M. P., Berezin A. S., Samsonenko D. G., Bagryanskaya I. Y., Brel V. K., Hei X., Brylev K. A., Artyushin O. I., Zelenkov L. E., Shishkin I. I., Li J. New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals // ACS applied materials & interfaces. 2022. Vol. 14. No. 27. pp. 31000-31009.
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TY - JOUR
DO - 10.1021/acsami.2c06438
UR - https://doi.org/10.1021/acsami.2c06438
TI - New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals
T2 - ACS applied materials & interfaces
AU - Artem'ev, Alexander V.
AU - Davydova, Maria P.
AU - Berezin, Alexey S
AU - Samsonenko, Denis G.
AU - Bagryanskaya, Irina Yu.
AU - Brel, Valery K.
AU - Hei, Xiuze
AU - Brylev, Konstantin A.
AU - Artyushin, Oleg I.
AU - Zelenkov, Lev E
AU - Shishkin, Ivan I
AU - Li, Jing
PY - 2022
DA - 2022/06/27
PB - American Chemical Society (ACS)
SP - 31000-31009
IS - 27
VL - 14
PMID - 35758694
SN - 1944-8244
SN - 1944-8252
ER -
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BibTex (до 50 авторов)
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@article{2022_Artem'ev,
author = {Alexander V. Artem'ev and Maria P. Davydova and Alexey S Berezin and Denis G. Samsonenko and Irina Yu. Bagryanskaya and Valery K. Brel and Xiuze Hei and Konstantin A. Brylev and Oleg I. Artyushin and Lev E Zelenkov and Ivan I Shishkin and Jing Li},
title = {New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals},
journal = {ACS applied materials & interfaces},
year = {2022},
volume = {14},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acsami.2c06438},
number = {27},
pages = {31000--31009},
doi = {10.1021/acsami.2c06438}
}
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MLA
Скопировать
Artem'ev, Alexander V., et al. “New Approach toward Dual-Emissive Organic–Inorganic Hybrids by Integrating Mn(II) and Cu(I) Emission Centers in Ionic Crystals.” ACS applied materials & interfaces, vol. 14, no. 27, Jun. 2022, pp. 31000-31009. https://doi.org/10.1021/acsami.2c06438.