Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media
G. L. Starova
1
,
Galina L Starova
1
,
Тип публикации: Journal Article
Дата публикации: 2019-12-20
scimago Q1
wos Q1
БС1
SJR: 0.981
CiteScore: 6.9
Impact factor: 4.7
ISSN: 26376105
Organic Chemistry
Process Chemistry and Technology
Polymers and Plastics
Краткое описание
In this work, we report on the synthesis of the two highly thermosensitive Eu complexes ([(tta)3Eu(NN1)] (Eu1) and [(tta)3Eu(NN2)] (Eu2), where tta is thenoyltrifluoroacetone, NN1 is 3-phenyl-2-(pyridin-2-yl)pyrido[2,1-a]pyrrolo[3,2-c]isoquinoline, and NN2 is 1-phenyl-2-(pyridin-2-yl)-1H-phenanthro[9,10-d]imidazole), and preparation of luminescent thermosensitive nanomaterial (latex nanothermometer, LNT). LNT design and preparation were based on the application of Eu2 and copolymerization of butyl and methyl methacrylates in the presence of the complex, surfactant (cetyltrimethylammonium bromide), and cosurfactant (acetone). Optimization of nanoemulsion polymerization conditions allowed us to obtain strongly luminescent nanoparticles with a narrow size distribution (D = 75 nm; PDI = 0.05). Moreover, the resulting LNT particles feature nonuniform distribution of Eu2, which localizes mainly inside the nanoparticles while the outer layer lacks the complex. As a result, the developed LNT demonstrates monoexpo...
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Shakirova J. R. et al. Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media // ACS Applied Polymer Materials. 2019. Vol. 2. No. 2. pp. 537-547.
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Shakirova J. R., Shevchenko N., Baigildin V. A., Chelushkin P. S., Khlebnikov A. F., Tomashenko O. A., Solomatina A. I., Starova G. L., Starova G. L., Tunik S. P. Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media // ACS Applied Polymer Materials. 2019. Vol. 2. No. 2. pp. 537-547.
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TY - JOUR
DO - 10.1021/acsapm.9b00952
UR - https://pubs.acs.org/doi/10.1021/acsapm.9b00952
TI - Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media
T2 - ACS Applied Polymer Materials
AU - Shakirova, Julia R
AU - Shevchenko, Natalia
AU - Baigildin, Vadim A.
AU - Chelushkin, Pavel S
AU - Khlebnikov, Alexander F
AU - Tomashenko, Olesya A
AU - Solomatina, Anastasia I
AU - Starova, G. L.
AU - Starova, Galina L
AU - Tunik, Sergey P.
PY - 2019
DA - 2019/12/20
PB - American Chemical Society (ACS)
SP - 537-547
IS - 2
VL - 2
SN - 2637-6105
ER -
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@article{2019_Shakirova,
author = {Julia R Shakirova and Natalia Shevchenko and Vadim A. Baigildin and Pavel S Chelushkin and Alexander F Khlebnikov and Olesya A Tomashenko and Anastasia I Solomatina and G. L. Starova and Galina L Starova and Sergey P. Tunik},
title = {Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media},
journal = {ACS Applied Polymer Materials},
year = {2019},
volume = {2},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://pubs.acs.org/doi/10.1021/acsapm.9b00952},
number = {2},
pages = {537--547},
doi = {10.1021/acsapm.9b00952}
}
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MLA
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Shakirova, Julia R., et al. “Eu-Based Phosphorescence Lifetime Polymer Nanothermometer: A Nanoemulsion Polymerization Approach to Eliminate Quenching of Eu Emission in Aqueous Media.” ACS Applied Polymer Materials, vol. 2, no. 2, Dec. 2019, pp. 537-547. https://pubs.acs.org/doi/10.1021/acsapm.9b00952.
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