Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light
Ting-Ting Hou
1, 2
,
Nengchao Luo
1, 2
,
Hongji Li
1, 2
,
Marc Heggen
3
,
Jian-Min Lu
1
,
YEHONG WANG
1
,
Feng Wang
1
3
Ernst
Ruska Centre for Microscopy and Spectroscopy with Electrons and Peter
Grünberg Institute, Forschungszentrum Juelich GmbH, Juelich 52425, Germany
|
Publication type: Journal Article
Publication date: 2017-05-10
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Abstract
Selective cleavage of C–C bonds is pursued as a useful chemical transformation method in biomass utilization. Herein, we report a hybrid CuOx/ceria/anatase nanotube catalyst in the selective oxidation of C–C bonds under visible light irradiation. Using the lignin β-1 model as a substrate offers 96% yields of benzaldehydes. Characterization results by high angle annular dark field scanning transmission electron microscopy (HAADF-STEM) and energy-dispersive X-ray spectroscopy element (EDX) mapping reveal that CuOx clusters are highly dispersed on the exposed anatase surface as well as on the nanosized ceria domains. In-depth investigations by Raman and ultraviolet visible diffuse reflectance spectra (UV−vis DRS), together with density functional theory (DFT) calculations, further verify that the CuOx clusters present on the ceria domains increase the concentration of surface defects (Ce3+ ions and oxygen vacancies) and accordingly improve the photocatalytic activity (Yang character); the CuOx clusters decor...
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Metrics
138
Total citations:
138
Citations from 2024:
43
(31.16%)
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GOST
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Hou T. et al. Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light // ACS Catalysis. 2017. Vol. 7. No. 6. pp. 3850-3859.
GOST all authors (up to 50)
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Hou T., Luo N., Li H., Heggen M., Lu J., WANG Y., Wang F. Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light // ACS Catalysis. 2017. Vol. 7. No. 6. pp. 3850-3859.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acscatal.7b00629
UR - https://doi.org/10.1021/acscatal.7b00629
TI - Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light
T2 - ACS Catalysis
AU - Hou, Ting-Ting
AU - Luo, Nengchao
AU - Li, Hongji
AU - Heggen, Marc
AU - Lu, Jian-Min
AU - WANG, YEHONG
AU - Wang, Feng
PY - 2017
DA - 2017/05/10
PB - American Chemical Society (ACS)
SP - 3850-3859
IS - 6
VL - 7
SN - 2155-5435
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Hou,
author = {Ting-Ting Hou and Nengchao Luo and Hongji Li and Marc Heggen and Jian-Min Lu and YEHONG WANG and Feng Wang},
title = {Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light},
journal = {ACS Catalysis},
year = {2017},
volume = {7},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acscatal.7b00629},
number = {6},
pages = {3850--3859},
doi = {10.1021/acscatal.7b00629}
}
Cite this
MLA
Copy
Hou, Ting-Ting, et al. “Yin and Yang Dual Characters of CuOx Clusters for C–C Bond Oxidation Driven by Visible Light.” ACS Catalysis, vol. 7, no. 6, May. 2017, pp. 3850-3859. https://doi.org/10.1021/acscatal.7b00629.