, volume 7 , issue 6 , pages 3860-3863

Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (T_g) Modulation

Nicole Kindermann ¹

Àlex Cristòfol ¹

Arjan W Kleij ^{1, 2}

Hide authors affiliations Show authors affiliations: 2 affiliations

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology (BIST), Av. Països Catalans 16, 43007 − Tarragona, Spain

Barcelona Institute for Science and Technology

Institute of Chemical Research of Catalonia

Catalan Institute of Research and Advanced Studies (ICREA), Pg. Lluís Companys 23, 08010 − Barcelona, Spain |

Publication type: Journal Article

Publication date: 2017-05-02

American Chemical Society (ACS)

ACS Catalysis

scimago Q1

wos Q1

SJR: 3.782

CiteScore: 19.5

Impact factor: 13.1

ISSN: 21555435

DOI: 10.1021/acscatal.7b00770

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General Chemistry

Catalysis

Abstract

A sequential and mild approach toward the synthesis of poly(limonene)dicarbonate (PLDC) has been developed using readily available limonene oxide (LO) and CO2 as renewable reagents and an air-stable Al(III) complex as catalyst for the alkene-rich poly(limonene)carbonate (PLC). The developed sequence allows for the stepwise construction of different PLDC polymers, using PLC as a synthetic intermediate with molecular weights of up to 15.3 kg/mol and tunable glass-transition temperature (Tg) values of up to an unprecedented 180 °C using a commercially available mixture of cis/trans (+)-LO.

Found

2 citations

Marta Elena

🥼 🤝

153 publications, 2 207 citations, 61 reviews

h-index: 24

Universidad de Alcalá

Research interests

Catalysis

Coordination Chemistry

Organometallic Chemistry

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Cite this

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GOST Copy

Kindermann N. et al. Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (Tg) Modulation // ACS Catalysis. 2017. Vol. 7. No. 6. pp. 3860-3863.

GOST all authors (up to 50) Copy

Kindermann N., Cristòfol À., Kleij A. W. Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (Tg) Modulation // ACS Catalysis. 2017. Vol. 7. No. 6. pp. 3860-3863.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acscatal.7b00770

UR - https://doi.org/10.1021/acscatal.7b00770

TI - Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (Tg) Modulation

T2 - ACS Catalysis

AU - Kindermann, Nicole

AU - Cristòfol, Àlex

AU - Kleij, Arjan W

PY - 2017

DA - 2017/05/02

PB - American Chemical Society (ACS)

SP - 3860-3863

IS - 6

VL - 7

SN - 2155-5435

ER -

BibTex |

Cite this

BibTex (up to 50 authors) Copy

@article{2017_Kindermann,

author = {Nicole Kindermann and Àlex Cristòfol and Arjan W Kleij},

title = {Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (Tg) Modulation},

journal = {ACS Catalysis},

year = {2017},

volume = {7},

publisher = {American Chemical Society (ACS)},

month = {may},

url = {https://doi.org/10.1021/acscatal.7b00770},

number = {6},

pages = {3860--3863},

doi = {10.1021/acscatal.7b00770}

}

MLA

Cite this

MLA Copy

Kindermann, Nicole, et al. “Access to Biorenewable Polycarbonates with Unusual Glass-Transition Temperature (Tg) Modulation.” ACS Catalysis, vol. 7, no. 6, May. 2017, pp. 3860-3863. https://doi.org/10.1021/acscatal.7b00770.

Publisher

American Chemical Society (ACS)

Journal

ACS Catalysis

scimago Q1

wos Q1

SJR

3.782

CiteScore

19.5

Impact factor

13.1

ISSN

21555435 (Print, Electronic)