Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope
1
Publication type: Journal Article
Publication date: 2017-12-22
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Abstract
The synergistic control of the SH2 transition states of hydrogen abstraction by polar and steric effects provides a promising strategy in achieving site-selective C(sp3)–H functionalization under decatungstate anion photocatalysis. By using this photocatalytic approach, the C–H bonds of alkanes, alcohols, ethers, ketones, amides, esters, nitriles, and pyridylalkanes were functionalized site-selectively. In the remarkable case of a 2,4-disubstituted cyclohexanone bearing five methyl, five methylene, and three methine C–H bonds, one methine C–H bond in the isoamyl tether was selectively functionalized.
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Ravelli D. et al. Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope // ACS Catalysis. 2017. Vol. 8. No. 1. pp. 701-713.
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Ravelli D., Fagnoni M., Fukuyama T., Nishikawa T., Ryu I. Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope // ACS Catalysis. 2017. Vol. 8. No. 1. pp. 701-713.
Cite this
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TY - JOUR
DO - 10.1021/acscatal.7b03354
UR - https://doi.org/10.1021/acscatal.7b03354
TI - Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope
T2 - ACS Catalysis
AU - Ravelli, Davide
AU - Fagnoni, Maurizio
AU - Fukuyama, Takahide
AU - Nishikawa, Tomohiro
AU - Ryu, Ilhyong
PY - 2017
DA - 2017/12/22
PB - American Chemical Society (ACS)
SP - 701-713
IS - 1
VL - 8
SN - 2155-5435
ER -
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BibTex (up to 50 authors)
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@article{2017_Ravelli,
author = {Davide Ravelli and Maurizio Fagnoni and Takahide Fukuyama and Tomohiro Nishikawa and Ilhyong Ryu},
title = {Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope},
journal = {ACS Catalysis},
year = {2017},
volume = {8},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acscatal.7b03354},
number = {1},
pages = {701--713},
doi = {10.1021/acscatal.7b03354}
}
Cite this
MLA
Copy
Ravelli, Davide, et al. “Site-Selective C–H Functionalization by Decatungstate Anion Photocatalysis: Synergistic Control by Polar and Steric Effects Expands the Reaction Scope.” ACS Catalysis, vol. 8, no. 1, Dec. 2017, pp. 701-713. https://doi.org/10.1021/acscatal.7b03354.