volume 8 issue 9 pages 8115-8120

Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis

Publication typeJournal Article
Publication date2018-07-17
scimago Q1
wos Q1
SJR3.782
CiteScore19.5
Impact factor13.1
ISSN21555435
General Chemistry
Catalysis
Abstract
A non-noble metal-free protocol has been developed for C–H bond functionalization at room temperature by merging cobalt-mediated catalysis with photocatalysis. The reaction requires only oxygen as sole oxidant and operated at room temperature under redox-neutral conditions. Visible-light activated photoredox catalyst functions as an electron transfer reagent with oxygen as a terminal oxidant in the cobalt-mediated C–H and N–H bond annulation. The developed methodology allows annulations with various coupling partners. The concept demonstrated herein is expected to enhance the scope of cobalt catalysis as applied to sustainable fine chemical synthesis.
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GOST |
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GOST Copy
Kalsi D. et al. Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis // ACS Catalysis. 2018. Vol. 8. No. 9. pp. 8115-8120.
GOST all authors (up to 50) Copy
Kalsi D., Dutta S., Barsu N., Rueping M., Sundararaju B. Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis // ACS Catalysis. 2018. Vol. 8. No. 9. pp. 8115-8120.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/acscatal.8b02118
UR - https://doi.org/10.1021/acscatal.8b02118
TI - Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis
T2 - ACS Catalysis
AU - Kalsi, Deepti
AU - Dutta, Subhradeep
AU - Barsu, Nagaraju
AU - Rueping, Magnus
AU - Sundararaju, Basker
PY - 2018
DA - 2018/07/17
PB - American Chemical Society (ACS)
SP - 8115-8120
IS - 9
VL - 8
SN - 2155-5435
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2018_Kalsi,
author = {Deepti Kalsi and Subhradeep Dutta and Nagaraju Barsu and Magnus Rueping and Basker Sundararaju},
title = {Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis},
journal = {ACS Catalysis},
year = {2018},
volume = {8},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/acscatal.8b02118},
number = {9},
pages = {8115--8120},
doi = {10.1021/acscatal.8b02118}
}
MLA
Cite this
MLA Copy
Kalsi, Deepti, et al. “Room-Temperature C–H Bond Functionalization by Merging Cobalt and Photoredox Catalysis.” ACS Catalysis, vol. 8, no. 9, Jul. 2018, pp. 8115-8120. https://doi.org/10.1021/acscatal.8b02118.