Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines
Тип публикации: Journal Article
Дата публикации: 2018-08-21
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 3.541
CiteScore: 20.4
Impact factor: 13.6
ISSN: 21555435
General Chemistry
Catalysis
Краткое описание
Highly enantioselective intramolecular RC reactions via desymmetrization of cyclohexadienones have been developed. By employing cyclohexadienones with a flexible ether or alkyl group linked internal enone moiety, optically enriched bicyclic pyran and hydrindane skeletons were constructed. Bifunctional phosphine catalysts bearing a thiourea moiety were found to effectively promote the reaction, and preliminary studies suggest that the hydrogen-bonding interaction between thiourea and carbonyl group is crucial and facilitates the otherwise flexible backbones to undergo the desired cyclization.
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Метрики
71
Всего цитирований:
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(11.26%)
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ГОСТ
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Li K. et al. Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines // ACS Catalysis. 2018. Vol. 8. No. 9. pp. 8810-8815.
ГОСТ со всеми авторами (до 50)
Скопировать
Li K., Jin Z., Chan W. L., Lu Y. Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines // ACS Catalysis. 2018. Vol. 8. No. 9. pp. 8810-8815.
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TY - JOUR
DO - 10.1021/acscatal.8b02706
UR - https://doi.org/10.1021/acscatal.8b02706
TI - Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines
T2 - ACS Catalysis
AU - Li, Kaizhi
AU - Jin, Zhichao
AU - Chan, Wai Lun
AU - Lu, Yixin
PY - 2018
DA - 2018/08/21
PB - American Chemical Society (ACS)
SP - 8810-8815
IS - 9
VL - 8
SN - 2155-5435
ER -
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BibTex (до 50 авторов)
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@article{2018_Li,
author = {Kaizhi Li and Zhichao Jin and Wai Lun Chan and Yixin Lu},
title = {Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines},
journal = {ACS Catalysis},
year = {2018},
volume = {8},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acscatal.8b02706},
number = {9},
pages = {8810--8815},
doi = {10.1021/acscatal.8b02706}
}
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MLA
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Li, Kaizhi, et al. “Enantioselective Construction of Bicyclic Pyran and Hydrindane Scaffolds via Intramolecular Rauhut–Currier Reactions Catalyzed by Thiourea-Phosphines.” ACS Catalysis, vol. 8, no. 9, Aug. 2018, pp. 8810-8815. https://doi.org/10.1021/acscatal.8b02706.
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