Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange
Manuel Kolb
3
,
Reshma Rao
3
,
Rasmus Frydendal
4
,
Fazal Raziq
5
,
X Renshaw Wang
6
,
Niels Bendtsen Halck
7
,
Jan Rossmeisl
8
,
Heine A. Hansen
7
,
Tejs Vegge
7
,
Ifan E. L. Stephens
3, 4
,
Marc T. Koper
2
,
Yang Shao-Horn
1, 3, 6
Publication type: Journal Article
Publication date: 2017-03-20
scimago Q1
wos Q1
SJR: 6.799
CiteScore: 29.6
Impact factor: 18.2
ISSN: 23808195
Materials Chemistry
Chemistry (miscellaneous)
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Abstract
RuO2 catalysts exhibit record activities toward the oxygen evolution reaction (OER), which is crucial to enable efficient and sustainable energy storage. Here we examine the RuO2 OER kinetics on rutile (110), (100), (101), and (111) orientations, finding (100) the most active. We assess the potential involvement of lattice oxygen in the OER mechanism with online electrochemical mass spectrometry, which showed no evidence of oxygen exchange on these oriented facets in acidic or basic electrolytes. Similar results were obtained for polyoriented RuO2 films and particles, in contrast to previous work, suggesting lattice oxygen is not exchanged in catalyzing OER on crystalline RuO2 surfaces. This hypothesis is supported by the correlation of activity with the number of active Ru-sites calculated by density functional theory, where more active facets bind oxygen more weakly. This new understanding of the active sites provides a design strategy to enhance the OER activity of RuO2 nanoparticles by facet engineering.
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Total citations:
348
Citations from 2024:
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(30.17%)
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Stoerzinger K. A. et al. Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange // ACS Energy Letters. 2017. Vol. 2. No. 4. pp. 876-881.
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Stoerzinger K. A., Diaz‐Morales O., Kolb M., Rao R., Frydendal R., Raziq F., Renshaw Wang X., Halck N. B., Rossmeisl J., Hansen H. A., Vegge T., Stephens I. E. L., Koper M. T., Shao-Horn Y. Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange // ACS Energy Letters. 2017. Vol. 2. No. 4. pp. 876-881.
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TY - JOUR
DO - 10.1021/acsenergylett.7b00135
UR - https://doi.org/10.1021/acsenergylett.7b00135
TI - Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange
T2 - ACS Energy Letters
AU - Stoerzinger, Kelsey A.
AU - Diaz‐Morales, Oscar
AU - Kolb, Manuel
AU - Rao, Reshma
AU - Frydendal, Rasmus
AU - Raziq, Fazal
AU - Renshaw Wang, X
AU - Halck, Niels Bendtsen
AU - Rossmeisl, Jan
AU - Hansen, Heine A.
AU - Vegge, Tejs
AU - Stephens, Ifan E. L.
AU - Koper, Marc T.
AU - Shao-Horn, Yang
PY - 2017
DA - 2017/03/20
PB - American Chemical Society (ACS)
SP - 876-881
IS - 4
VL - 2
SN - 2380-8195
ER -
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BibTex (up to 50 authors)
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@article{2017_Stoerzinger,
author = {Kelsey A. Stoerzinger and Oscar Diaz‐Morales and Manuel Kolb and Reshma Rao and Rasmus Frydendal and Fazal Raziq and X Renshaw Wang and Niels Bendtsen Halck and Jan Rossmeisl and Heine A. Hansen and Tejs Vegge and Ifan E. L. Stephens and Marc T. Koper and Yang Shao-Horn},
title = {Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange},
journal = {ACS Energy Letters},
year = {2017},
volume = {2},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acsenergylett.7b00135},
number = {4},
pages = {876--881},
doi = {10.1021/acsenergylett.7b00135}
}
Cite this
MLA
Copy
Stoerzinger, Kelsey A., et al. “Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange.” ACS Energy Letters, vol. 2, no. 4, Mar. 2017, pp. 876-881. https://doi.org/10.1021/acsenergylett.7b00135.