Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst
Publication type: Journal Article
Publication date: 2015-04-30
scimago Q1
wos Q1
SJR: 1.287
CiteScore: 8.9
Impact factor: 5.2
ISSN: 21611653
PubMed ID:
35596283
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
Living radical polymerization of acrylates and acrylamides from trithiocarbonate iniferters using a compact fluorescent lamp (CFL) bulb and 10-phenylphenothiazine as an organic photoredox catalyst is reported. With this system, chain growth can be efficiently switched between "on" and "off" in response to visible light. Polymer molar masses increase linearly with conversion, and narrow molar mass distributions are obtained. The excellent fidelity of the trithiocarbonate-iniferter enables the preparation of triblock copolymers from macro-iniferters under the same visible-light mediated protocol, using UV light without a photoredox catalyst or under traditional thermally induced RAFT conditions. We expect that the simplicity and efficiency of this metal-free, visible-light-mediated polymerization will enable the synthesis and modification of a range of materials under mild conditions.
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208
Total citations:
208
Citations from 2024:
17
(8.18%)
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Chen M., Macleod M. J., Johnson J. N. Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst // ACS Macro Letters. 2015. Vol. 4. No. 5. pp. 566-569.
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Chen M., Macleod M. J., Johnson J. N. Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst // ACS Macro Letters. 2015. Vol. 4. No. 5. pp. 566-569.
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RIS
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TY - JOUR
DO - 10.1021/acsmacrolett.5b00241
UR - https://doi.org/10.1021/acsmacrolett.5b00241
TI - Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst
T2 - ACS Macro Letters
AU - Chen, Mao
AU - Macleod, Michelle J
AU - Johnson, Jeremiah N.
PY - 2015
DA - 2015/04/30
PB - American Chemical Society (ACS)
SP - 566-569
IS - 5
VL - 4
PMID - 35596283
SN - 2161-1653
ER -
Cite this
BibTex (up to 50 authors)
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@article{2015_Chen,
author = {Mao Chen and Michelle J Macleod and Jeremiah N. Johnson},
title = {Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst},
journal = {ACS Macro Letters},
year = {2015},
volume = {4},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acsmacrolett.5b00241},
number = {5},
pages = {566--569},
doi = {10.1021/acsmacrolett.5b00241}
}
Cite this
MLA
Copy
Chen, Mao, et al. “Visible-Light-Controlled Living Radical Polymerization from a Trithiocarbonate Iniferter Mediated by an Organic Photoredox Catalyst.” ACS Macro Letters, vol. 4, no. 5, Apr. 2015, pp. 566-569. https://doi.org/10.1021/acsmacrolett.5b00241.