Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization
Zhanhua Wang
1, 2
,
Zhanhua Wang
1
,
Xiangcheng Pan
3
,
Li-ye Fu
2
,
Sushil Lathwal
2
,
Mateusz Olszewski
2
,
Jiajun Yan
2
,
Alan Enciso
2
,
Zongyu Wang
2
,
Hesheng Xia
1
,
Krzysztof Matyjaszewski
2
Publication type: Journal Article
Publication date: 2018-02-16
scimago Q1
wos Q1
SJR: 1.287
CiteScore: 8.9
Impact factor: 5.2
ISSN: 21611653
PubMed ID:
35632917
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
A new procedure for ultrasonication-induced atom transfer radical polymerization (sono-ATRP) in aqueous media was developed. Polymerizations of oligo(ethylene oxide) methyl ether methacrylate (OEOMA) and 2-hydroxyethyl acrylate (HEA) in water were successfully carried out in the presence of ppm amounts of CuBr2 catalyst and tris(2-pyridylmethyl)amine ligand when exposed to ultrasonication (40 kHz, 110 W) at room temperature. Aqueous sono-ATRP enabled polymerization of water-soluble monomers with excellent control over the molecular weight, dispersity, and high retention of chain-end functionality. Temporal control over the polymer chain growth was demonstrated by switching the ultrasound on/off due to the regeneration of activators by hydroxyl radicals formed by ultrasonication. The synthesis of a well-defined block copolymer and DNA-polymer biohybrid was also successful using this process.
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148
Total citations:
148
Citations from 2024:
28
(19.04%)
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GOST
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Wang Z. et al. Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization // ACS Macro Letters. 2018. Vol. 7. No. 3. pp. 275-280.
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Wang Z., Wang Z., Pan X., Fu L., Lathwal S., Olszewski M., Yan J., Enciso A., Wang Z., Xia H., Matyjaszewski K. Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization // ACS Macro Letters. 2018. Vol. 7. No. 3. pp. 275-280.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acsmacrolett.8b00027
UR - https://doi.org/10.1021/acsmacrolett.8b00027
TI - Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization
T2 - ACS Macro Letters
AU - Wang, Zhanhua
AU - Wang, Zhanhua
AU - Pan, Xiangcheng
AU - Fu, Li-ye
AU - Lathwal, Sushil
AU - Olszewski, Mateusz
AU - Yan, Jiajun
AU - Enciso, Alan
AU - Wang, Zongyu
AU - Xia, Hesheng
AU - Matyjaszewski, Krzysztof
PY - 2018
DA - 2018/02/16
PB - American Chemical Society (ACS)
SP - 275-280
IS - 3
VL - 7
PMID - 35632917
SN - 2161-1653
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Wang,
author = {Zhanhua Wang and Zhanhua Wang and Xiangcheng Pan and Li-ye Fu and Sushil Lathwal and Mateusz Olszewski and Jiajun Yan and Alan Enciso and Zongyu Wang and Hesheng Xia and Krzysztof Matyjaszewski},
title = {Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization},
journal = {ACS Macro Letters},
year = {2018},
volume = {7},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/acsmacrolett.8b00027},
number = {3},
pages = {275--280},
doi = {10.1021/acsmacrolett.8b00027}
}
Cite this
MLA
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Wang, Zhanhua, et al. “Ultrasonication-Induced Aqueous Atom Transfer Radical Polymerization.” ACS Macro Letters, vol. 7, no. 3, Feb. 2018, pp. 275-280. https://doi.org/10.1021/acsmacrolett.8b00027.