ACS Nano, volume 9, issue 7, pages 7151-7163

Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange

Jian Zhang ^{1, 2}

Boris D Chernomordik ²

Ryan Patrick Crisp ^{2, 3}

Daniel M Kroupa ^{2, 4}

Joseph M. Luther ²

Elisa M. Miller ²

Yamei Liu ⁵

Matthew C Beard ²

Hide authors affiliations Show authors affiliations: 5 affiliations

School of Optical and Electronic Information, Huazhong University of Science and Technology, Hubei 430074, China |

Chemical and Material Sciences Center, National Renewable Energy Laboratory, Golden, Colorado 80401, United States |

Department of Physics, Colorado School of Mines, Golden, Colorado 80401, United States |

⁴

Department of Chemistry and Biochemistry, University of Colorado, Boulder, Colorado 80309, United States |

⁵

Center for Advanced Solar Photophysics, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States |

Publication type: Journal Article

Publication date: 2015-07-17

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/acsnano.5b01859

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

We developed a strategy for producing quasi-spherical nanocrystals of anisotropic heterostructures of Cd/Pb chalcogenides. The nanostructures are fabricated via a controlled cation exchange reaction where the Cd(2+) cation is exchanged for the Pb(2+) cation. The cation exchange reaction is thermally activated and can be controlled by adjusting the reaction temperature or time. We characterized the particles using TEM, XPS, PL, and absorption spectroscopy. With complete exchange, high quality Pb-chalcogenide quantum dots are produced. In addition to Cd(2+), we also find suitable conditions for the exchange of Zn(2+) cations for Pb(2+) cations. The cation exchange is anisotropic starting at one edge of the nanocrystals and proceeds along the ⟨111⟩ direction producing a sharp interface at a (111) crystallographic plane. Instead of spherical core/shell structures, we produced and studied quasi-spherical CdS/PbS and CdSe/PbSe Janus-type heterostructures. Nontrivial PL behavior was observed from the CdS(e)/PbS(e) heterostructures as the Pb:Cd ratio is increased.

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Citations by journals

	2 4 6 8 10 12
Chemistry of Materials	Chemistry of Materials, 12, 12.24% Chemistry of Materials 12 publications, 12.24%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 7.14% Journal of Physical Chemistry C 7 publications, 7.14%
Journal of the American Chemical Society	Journal of the American Chemical Society, 4, 4.08% Journal of the American Chemical Society 4 publications, 4.08%
Nano Letters	Nano Letters, 4, 4.08% Nano Letters 4 publications, 4.08%
Nano Research	Nano Research, 3, 3.06% Nano Research 3 publications, 3.06%
Advanced Functional Materials	Advanced Functional Materials, 3, 3.06% Advanced Functional Materials 3 publications, 3.06%
ACS Nano	ACS Nano, 3, 3.06% ACS Nano 3 publications, 3.06%
Chemical Reviews	Chemical Reviews, 3, 3.06% Chemical Reviews 3 publications, 3.06%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 3.06% ACS applied materials & interfaces 3 publications, 3.06%
Langmuir	Langmuir, 3, 3.06% Langmuir 3 publications, 3.06%
ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 3.06% ACS Applied Nano Materials 3 publications, 3.06%
CrystEngComm	CrystEngComm, 3, 3.06% CrystEngComm 3 publications, 3.06%
Nature Communications	Nature Communications, 2, 2.04% Nature Communications 2 publications, 2.04%
Nano-Micro Letters	Nano-Micro Letters, 2, 2.04% Nano-Micro Letters 2 publications, 2.04%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 2, 2.04% Solar Energy Materials and Solar Cells 2 publications, 2.04%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 2, 2.04% Journal of Physical Chemistry Letters 2 publications, 2.04%
Nanoscale	Nanoscale, 2, 2.04% Nanoscale 2 publications, 2.04%
ACS Photonics	ACS Photonics, 1, 1.02% ACS Photonics 1 publication, 1.02%
Journal of Applied Physics	Journal of Applied Physics, 1, 1.02% Journal of Applied Physics 1 publication, 1.02%
Solar RRL	Solar RRL, 1, 1.02% Solar RRL 1 publication, 1.02%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 1, 1.02% Applied Sciences (Switzerland) 1 publication, 1.02%
Water (Switzerland)	Water (Switzerland), 1, 1.02% Water (Switzerland) 1 publication, 1.02%
Nature Electronics	Nature Electronics, 1, 1.02% Nature Electronics 1 publication, 1.02%
Nano Convergence	Nano Convergence, 1, 1.02% Nano Convergence 1 publication, 1.02%
Journal of Electronic Materials	Journal of Electronic Materials, 1, 1.02% Journal of Electronic Materials 1 publication, 1.02%
Journal of Semiconductors	Journal of Semiconductors, 1, 1.02% Journal of Semiconductors 1 publication, 1.02%
Sensors and Actuators, B: Chemical	Sensors and Actuators, B: Chemical, 1, 1.02% Sensors and Actuators, B: Chemical 1 publication, 1.02%
Talanta	Talanta, 1, 1.02% Talanta 1 publication, 1.02%
Accounts of Chemical Research	Accounts of Chemical Research, 1, 1.02% Accounts of Chemical Research 1 publication, 1.02%
	2 4 6 8 10 12

Citations by publishers

	5 10 15 20 25 30 35 40 45 50
American Chemical Society (ACS)	American Chemical Society (ACS), 48, 48.98% American Chemical Society (ACS) 48 publications, 48.98%
Springer Nature	Springer Nature, 12, 12.24% Springer Nature 12 publications, 12.24%
Elsevier	Elsevier, 10, 10.2% Elsevier 10 publications, 10.2%
Wiley	Wiley, 9, 9.18% Wiley 9 publications, 9.18%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 7, 7.14% Royal Society of Chemistry (RSC) 7 publications, 7.14%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 2.04% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 2.04%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 1.02% American Institute of Physics (AIP) 1 publication, 1.02%
IOP Publishing	IOP Publishing, 1, 1.02% IOP Publishing 1 publication, 1.02%
Taylor & Francis	Taylor & Francis, 1, 1.02% Taylor & Francis 1 publication, 1.02%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 1.02% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 1.02%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.02% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.02%
	5 10 15 20 25 30 35 40 45 50

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GOST Copy

Zhang J. et al. Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange // ACS Nano. 2015. Vol. 9. No. 7. pp. 7151-7163.

GOST all authors (up to 50) Copy

Zhang J., Chernomordik B. D., Crisp R. P., Kroupa D. M., Luther J. M., Miller E. M., Liu Y., Beard M. C. Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange // ACS Nano. 2015. Vol. 9. No. 7. pp. 7151-7163.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acsnano.5b01859

UR - https://doi.org/10.1021/acsnano.5b01859

TI - Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange

T2 - ACS Nano

AU - Chernomordik, Boris D

AU - Zhang, Jian

AU - Crisp, Ryan Patrick

AU - Kroupa, Daniel M

AU - Luther, Joseph M.

AU - Miller, Elisa M.

AU - Liu, Yamei

AU - Beard, Matthew C

PY - 2015

DA - 2015/07/17 00:00:00

PB - American Chemical Society (ACS)

SP - 7151-7163

IS - 7

VL - 9

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

Cite this

BibTex Copy

@article{2015_Zhang,

author = {Boris D Chernomordik and Jian Zhang and Ryan Patrick Crisp and Daniel M Kroupa and Joseph M. Luther and Elisa M. Miller and Yamei Liu and Matthew C Beard},

title = {Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange},

journal = {ACS Nano},

year = {2015},

volume = {9},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://doi.org/10.1021/acsnano.5b01859},

number = {7},

pages = {7151--7163},

doi = {10.1021/acsnano.5b01859}

}

MLA

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MLA Copy

Zhang, Jian, et al. “Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange.” ACS Nano, vol. 9, no. 7, Jul. 2015, pp. 7151-7163. https://doi.org/10.1021/acsnano.5b01859.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)