ACS Nano, volume 9, issue 9, pages 8833-8842

Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression

Alex Ip ¹

Amirreza Kiani ¹

Illan J Kramer ¹

Oleksandr Voznyy ¹

Hamidreza F Movahed ¹

Larissa Levina ¹

Michael M Adachi ¹

Sjoerd Hoogland ¹

Edward H Sargent ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Department of Electrical and Computer Engineering, University of Toronto, 10 King’s College Road, Toronto, Ontario M5S 3G4, Canada |

Publication type: Journal Article

Publication date: 2015-08-19

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/acsnano.5b02164

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

Materials optimized for single-junction solar spectral harvesting, such as silicon, perovskites, and large-band-gap colloidal quantum dot solids, fail to absorb the considerable infrared spectral energy that lies below their respective band gap. Here we explore through modeling and experiment the potential for colloidal quantum dots (CQDs) to augment the performance of solar cells by harnessing transmitted light in the infrared. Through detailed balance modeling, we identify the CQD band gap that is best able to augment wafer-based, thin-film, and also solution-processed photovoltaic (PV) materials. The required quantum dots, with an excitonic peak at 1.3 μm, have not previously been studied in depth for solar performance. Using computational studies we find that a new ligand scheme distinct from that employed in better-explored 0.95 μm band gap PbS CQDs is necessary; only via the solution-phase application of a short bromothiol can we prevent dot fusion during ensuing solid-state film treatments and simultaneously offer a high valence band-edge density of states to enhance hole transport. Photoluminescence spectra and transient studies confirm the desired narrowed emission peaks and reduced surface-trap-associated decay. Electronic characterization reveals that only through the use of the bromothiol ligands is strong hole transport retained. The films, when used to make PV devices, achieve the highest AM1.5 power conversion efficiency yet reported in a solution-processed material having a sub-1 eV band gap.

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Citations by journals

	1 2 3 4 5 6 7 8 9
Advanced Materials	Advanced Materials, 9, 9.28% Advanced Materials 9 publications, 9.28%
ACS Energy Letters	ACS Energy Letters, 8, 8.25% ACS Energy Letters 8 publications, 8.25%
Small	Small, 4, 4.12% Small 4 publications, 4.12%
Nano Letters	Nano Letters, 4, 4.12% Nano Letters 4 publications, 4.12%
Nanoscale	Nanoscale, 4, 4.12% Nanoscale 4 publications, 4.12%
Advanced Functional Materials	Advanced Functional Materials, 3, 3.09% Advanced Functional Materials 3 publications, 3.09%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 3.09% ACS applied materials & interfaces 3 publications, 3.09%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 3, 3.09% Journal of Physical Chemistry Letters 3 publications, 3.09%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 2, 2.06% Applied Sciences (Switzerland) 2 publications, 2.06%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 2.06% Chemical Engineering Journal 2 publications, 2.06%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 2, 2.06% Journal of Materials Science and Technology 2 publications, 2.06%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 2, 2.06% Journal of Alloys and Compounds 2 publications, 2.06%
ACS Nano	ACS Nano, 2, 2.06% ACS Nano 2 publications, 2.06%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 2.06% Journal of Physical Chemistry C 2 publications, 2.06%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 2.06% Journal of the American Chemical Society 2 publications, 2.06%
Science	Science, 2, 2.06% Science 2 publications, 2.06%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 2.06% Journal of Materials Chemistry A 2 publications, 2.06%
Applied Physics Letters	Applied Physics Letters, 1, 1.03% Applied Physics Letters 1 publication, 1.03%
Chemical Physics Reviews	Chemical Physics Reviews, 1, 1.03% Chemical Physics Reviews 1 publication, 1.03%
Nano Research	Nano Research, 1, 1.03% Nano Research 1 publication, 1.03%
Nature Materials	Nature Materials, 1, 1.03% Nature Materials 1 publication, 1.03%
Nature Reviews Materials	Nature Reviews Materials, 1, 1.03% Nature Reviews Materials 1 publication, 1.03%
Multimedia Tools and Applications	Multimedia Tools and Applications, 1, 1.03% Multimedia Tools and Applications 1 publication, 1.03%
Nature Nanotechnology	Nature Nanotechnology, 1, 1.03% Nature Nanotechnology 1 publication, 1.03%
Nature Communications	Nature Communications, 1, 1.03% Nature Communications 1 publication, 1.03%
Ceramics International	Ceramics International, 1, 1.03% Ceramics International 1 publication, 1.03%
Optical Materials	Optical Materials, 1, 1.03% Optical Materials 1 publication, 1.03%
Journal of Electronic Science and Technology	Journal of Electronic Science and Technology, 1, 1.03% Journal of Electronic Science and Technology 1 publication, 1.03%
Journal of Molecular Structure	Journal of Molecular Structure, 1, 1.03% Journal of Molecular Structure 1 publication, 1.03%
Nanotechnology	Nanotechnology, 1, 1.03% Nanotechnology 1 publication, 1.03%
	1 2 3 4 5 6 7 8 9

Citations by publishers

	5 10 15 20 25 30
Wiley	Wiley, 27, 27.84% Wiley 27 publications, 27.84%
American Chemical Society (ACS)	American Chemical Society (ACS), 26, 26.8% American Chemical Society (ACS) 26 publications, 26.8%
Elsevier	Elsevier, 11, 11.34% Elsevier 11 publications, 11.34%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 11, 11.34% Royal Society of Chemistry (RSC) 11 publications, 11.34%
Springer Nature	Springer Nature, 8, 8.25% Springer Nature 8 publications, 8.25%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 2.06% American Institute of Physics (AIP) 2 publications, 2.06%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 2.06% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 2.06%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 2, 2.06% American Association for the Advancement of Science (AAAS) 2 publications, 2.06%
University of Electronic Science and Technology of China	University of Electronic Science and Technology of China, 1, 1.03% University of Electronic Science and Technology of China 1 publication, 1.03%
IOP Publishing	IOP Publishing, 1, 1.03% IOP Publishing 1 publication, 1.03%
American Physical Society (APS)	American Physical Society (APS), 1, 1.03% American Physical Society (APS) 1 publication, 1.03%
Walter de Gruyter	Walter de Gruyter, 1, 1.03% Walter de Gruyter 1 publication, 1.03%
Optical Society of America	Optical Society of America, 1, 1.03% Optical Society of America 1 publication, 1.03%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.03% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.03%
Taylor & Francis	Taylor & Francis, 1, 1.03% Taylor & Francis 1 publication, 1.03%
	5 10 15 20 25 30

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GOST Copy

Ip A. et al. Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression // ACS Nano. 2015. Vol. 9. No. 9. pp. 8833-8842.

GOST all authors (up to 50) Copy

Ip A., Kiani A., Kramer I. J., Voznyy O., Movahed H. F., Levina L., Adachi M. M., Hoogland S., Sargent E. H. Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression // ACS Nano. 2015. Vol. 9. No. 9. pp. 8833-8842.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acsnano.5b02164

UR - https://doi.org/10.1021/acsnano.5b02164

TI - Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression

T2 - ACS Nano

AU - Kiani, Amirreza

AU - Movahed, Hamidreza F

AU - Levina, Larissa

AU - Adachi, Michael M

AU - Ip, Alex

AU - Kramer, Illan J

AU - Voznyy, Oleksandr

AU - Hoogland, Sjoerd

AU - Sargent, Edward H

PY - 2015

DA - 2015/08/19 00:00:00

PB - American Chemical Society (ACS)

SP - 8833-8842

IS - 9

VL - 9

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

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BibTex Copy

@article{2015_Ip,

author = {Amirreza Kiani and Hamidreza F Movahed and Larissa Levina and Michael M Adachi and Alex Ip and Illan J Kramer and Oleksandr Voznyy and Sjoerd Hoogland and Edward H Sargent},

title = {Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression},

journal = {ACS Nano},

year = {2015},

volume = {9},

publisher = {American Chemical Society (ACS)},

month = {aug},

url = {https://doi.org/10.1021/acsnano.5b02164},

number = {9},

pages = {8833--8842},

doi = {10.1021/acsnano.5b02164}

}

MLA

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MLA Copy

Ip, Alex, et al. “Infrared Colloidal Quantum Dot PhotovoltaicsviaCoupling Enhancement and Agglomeration Suppression.” ACS Nano, vol. 9, no. 9, Aug. 2015, pp. 8833-8842. https://doi.org/10.1021/acsnano.5b02164.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)