ACS Nano, volume 10, issue 3, pages 3356-3364

Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals.

L. Biadala ¹

Benjamin Siebers ¹

Yasin Beyazit ¹

Mickael Tessier

Dorian Dupont

Zeger Hens

D G Yakovlev ^{1, 2}

M. Bayer ^{1, 2}

Hide authors affiliations Show authors affiliations: 2 affiliations

Experimentelle Physik 2, Technische Universität Dortmund, 44221 Dortmund, Germany |

Ioffe Institute, Russian Academy of Sciences, 194021 St. Petersburg, Russia |

Publication type: Journal Article

Publication date: 2016-02-24

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/acsnano.5b07065

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

We report on a temperature-, time-, and spectrally resolved study of the photoluminescence of type-I InP/ZnS colloidal nanocrystals with varying core size. By studying the exciton recombination dynamics we assess the exciton fine structure in these systems. In addition to the typical bright-dark doublet, the photoluminescence stems from an upper bright state in spite of its large energy splitting (∼100 meV). This striking observation results from dramatically lengthened thermalization processes among the fine structure levels and points to optical-phonon bottleneck effects in InP/ZnS nanocrystals. Furthermore, our data show that the radiative recombination of the dark exciton scales linearly with the bright-dark energy splitting for CdSe and InP nanocrystals. This finding strongly suggests a universal dangling bonds-assisted recombination of the dark exciton in colloidal nanostructures.

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ACS Nano	ACS Nano, 7, 10.14% ACS Nano 7 publications, 10.14%
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Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 5, 7.25% Journal of Physical Chemistry Letters 5 publications, 7.25%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 3, 4.35% Journal of Physical Chemistry C 3 publications, 4.35%
Journal of Chemical Physics	Journal of Chemical Physics, 3, 4.35% Journal of Chemical Physics 3 publications, 4.35%
Journal of Physics: Conference Series	Journal of Physics: Conference Series, 3, 4.35% Journal of Physics: Conference Series 3 publications, 4.35%
Physical Review B	Physical Review B, 2, 2.9% Physical Review B 2 publications, 2.9%
Scientific Reports	Scientific Reports, 2, 2.9% Scientific Reports 2 publications, 2.9%
Nature Communications	Nature Communications, 2, 2.9% Nature Communications 2 publications, 2.9%
Nanoscale Research Letters	Nanoscale Research Letters, 2, 2.9% Nanoscale Research Letters 2 publications, 2.9%
Journal of Luminescence	Journal of Luminescence, 2, 2.9% Journal of Luminescence 2 publications, 2.9%
Applied Surface Science	Applied Surface Science, 2, 2.9% Applied Surface Science 2 publications, 2.9%
Small	Small, 2, 2.9% Small 2 publications, 2.9%
Advanced Optical Materials	Advanced Optical Materials, 2, 2.9% Advanced Optical Materials 2 publications, 2.9%
ACS Photonics	ACS Photonics, 2, 2.9% ACS Photonics 2 publications, 2.9%
Chemical Reviews	Chemical Reviews, 2, 2.9% Chemical Reviews 2 publications, 2.9%
Nanoscale	Nanoscale, 2, 2.9% Nanoscale 2 publications, 2.9%
Physical Review Letters	Physical Review Letters, 1, 1.45% Physical Review Letters 1 publication, 1.45%
ACS Applied Nano Materials	ACS Applied Nano Materials, 1, 1.45% ACS Applied Nano Materials 1 publication, 1.45%
NPG Asia Materials	NPG Asia Materials, 1, 1.45% NPG Asia Materials 1 publication, 1.45%
Nature Photonics	Nature Photonics, 1, 1.45% Nature Photonics 1 publication, 1.45%
Applied Nanoscience (Switzerland)	Applied Nanoscience (Switzerland), 1, 1.45% Applied Nanoscience (Switzerland) 1 publication, 1.45%
Topics in Current Chemistry	Topics in Current Chemistry, 1, 1.45% Topics in Current Chemistry 1 publication, 1.45%
Korean Journal of Chemical Engineering	Korean Journal of Chemical Engineering, 1, 1.45% Korean Journal of Chemical Engineering 1 publication, 1.45%
Journal of Electronic Materials	Journal of Electronic Materials, 1, 1.45% Journal of Electronic Materials 1 publication, 1.45%
Solar RRL	Solar RRL, 1, 1.45% Solar RRL 1 publication, 1.45%
Journal of the American Chemical Society	Journal of the American Chemical Society, 1, 1.45% Journal of the American Chemical Society 1 publication, 1.45%
ACS Energy Letters	ACS Energy Letters, 1, 1.45% ACS Energy Letters 1 publication, 1.45%
Russian Chemical Bulletin	Russian Chemical Bulletin, 1, 1.45% Russian Chemical Bulletin 1 publication, 1.45%
Chemical Society Reviews	Chemical Society Reviews, 1, 1.45% Chemical Society Reviews 1 publication, 1.45%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25 30
American Chemical Society (ACS)	American Chemical Society (ACS), 28, 40.58% American Chemical Society (ACS) 28 publications, 40.58%
Springer Nature	Springer Nature, 13, 18.84% Springer Nature 13 publications, 18.84%
Elsevier	Elsevier, 5, 7.25% Elsevier 5 publications, 7.25%
Wiley	Wiley, 5, 7.25% Wiley 5 publications, 7.25%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 5.8% American Institute of Physics (AIP) 4 publications, 5.8%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 4, 5.8% Royal Society of Chemistry (RSC) 4 publications, 5.8%
American Physical Society (APS)	American Physical Society (APS), 3, 4.35% American Physical Society (APS) 3 publications, 4.35%
IOP Publishing	IOP Publishing, 3, 4.35% IOP Publishing 3 publications, 4.35%
Pleiades Publishing	Pleiades Publishing, 1, 1.45% Pleiades Publishing 1 publication, 1.45%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.45% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.45%
Annual Reviews	Annual Reviews, 1, 1.45% Annual Reviews 1 publication, 1.45%
	5 10 15 20 25 30

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Biadala L. et al. Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals. // ACS Nano. 2016. Vol. 10. No. 3. pp. 3356-3364.

GOST all authors (up to 50) Copy

Biadala L., Siebers B., Beyazit Y., Tessier M., Dupont D., Hens Z., Yakovlev D. G., Bayer M. Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals. // ACS Nano. 2016. Vol. 10. No. 3. pp. 3356-3364.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acsnano.5b07065

UR - https://doi.org/10.1021/acsnano.5b07065

TI - Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals.

T2 - ACS Nano

AU - Siebers, Benjamin

AU - Beyazit, Yasin

AU - Dupont, Dorian

AU - Biadala, L.

AU - Tessier, Mickael

AU - Hens, Zeger

AU - Yakovlev, D G

AU - Bayer, M.

PY - 2016

DA - 2016/02/24 00:00:00

PB - American Chemical Society (ACS)

SP - 3356-3364

IS - 3

VL - 10

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

Cite this

BibTex Copy

@article{2016_Biadala,

author = {Benjamin Siebers and Yasin Beyazit and Dorian Dupont and L. Biadala and Mickael Tessier and Zeger Hens and D G Yakovlev and M. Bayer},

title = {Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals.},

journal = {ACS Nano},

year = {2016},

volume = {10},

publisher = {American Chemical Society (ACS)},

month = {feb},

url = {https://doi.org/10.1021/acsnano.5b07065},

number = {3},

pages = {3356--3364},

doi = {10.1021/acsnano.5b07065}

}

MLA

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MLA Copy

Biadala, L., et al. “Band-Edge Exciton Fine Structure and Recombination Dynamics in InP/ZnS Colloidal Nanocrystals..” ACS Nano, vol. 10, no. 3, Feb. 2016, pp. 3356-3364. https://doi.org/10.1021/acsnano.5b07065.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)