ACS Nano, volume 12, issue 4, pages 3397-3405

Two Mechanisms Determine Quantum Dot Blinking.

Gangcheng Yuan ¹

Daniel E. Gómez ²

Nicholas Kirkwood ¹

Klaus Boldt ¹

Paul Mulvaney ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

ARC Centre of Excellence in Exciton Science, School of Chemistry, University of Melbourne, Parkville, Victoria 3010, Australia |

RMIT University, Melbourne, Victoria 3000, Australia |

Publication type: Journal Article

Publication date: 2018-03-26

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/acsnano.7b09052

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

Many potential applications of quantum dots (QDs) can only be realized once the luminescence from single nanocrystals (NCs) is understood. These applications include the development of quantum logic devices, single-photon sources, long-life LEDs, and single-molecule biolabels. At the single-nanocrystal level, random fluctuations in the QD photoluminescence occur, a phenomenon termed blinking. There are two competing models to explain this blinking: Auger recombination and surface trap induced recombination. Here we use lifetime scaling on core-shell chalcogenide NCs to demonstrate that both types of blinking occur in the same QDs. We prove that Auger-blinking can yield single-exponential on/off times in contrast to earlier work. The surface passivation strategy determines which blinking mechanism dominates. This study summarizes earlier studies on blinking mechanisms and provides some clues that stable single QDs can be engineered for optoelectronic applications.

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Optics and Spectroscopy (English translation of Optika i Spektroskopiya)	Optics and Spectroscopy (English translation of Optika i Spektroskopiya), 3, 1.84% Optics and Spectroscopy (English translation of Optika i Spektroskopiya) 3 publications, 1.84%
Acta Physica Sinica	Acta Physica Sinica, 3, 1.84% Acta Physica Sinica 3 publications, 1.84%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 1.84% Journal of Materials Chemistry C 3 publications, 1.84%
Journal of Luminescence	Journal of Luminescence, 2, 1.23% Journal of Luminescence 2 publications, 1.23%
Nanomaterials	Nanomaterials, 2, 1.23% Nanomaterials 2 publications, 1.23%
Advanced Photonics Research	Advanced Photonics Research, 2, 1.23% Advanced Photonics Research 2 publications, 1.23%
ACS Applied Nano Materials	ACS Applied Nano Materials, 2, 1.23% ACS Applied Nano Materials 2 publications, 1.23%
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Small Science	Small Science, 2, 1.23% Small Science 2 publications, 1.23%
ChemPhysChem	ChemPhysChem, 1, 0.61% ChemPhysChem 1 publication, 0.61%
APL Materials	APL Materials, 1, 0.61% APL Materials 1 publication, 0.61%
AVS Quantum Science	AVS Quantum Science, 1, 0.61% AVS Quantum Science 1 publication, 0.61%
International Journal of Molecular Sciences	International Journal of Molecular Sciences, 1, 0.61% International Journal of Molecular Sciences 1 publication, 0.61%
Nature Communications	Nature Communications, 1, 0.61% Nature Communications 1 publication, 0.61%
Frontiers of Physics	Frontiers of Physics, 1, 0.61% Frontiers of Physics 1 publication, 0.61%
	5 10 15 20 25

Citations by publishers

	10 20 30 40 50 60 70 80
American Chemical Society (ACS)	American Chemical Society (ACS), 72, 44.17% American Chemical Society (ACS) 72 publications, 44.17%
Wiley	Wiley, 24, 14.72% Wiley 24 publications, 14.72%
Springer Nature	Springer Nature, 15, 9.2% Springer Nature 15 publications, 9.2%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 12, 7.36% Royal Society of Chemistry (RSC) 12 publications, 7.36%
Elsevier	Elsevier, 8, 4.91% Elsevier 8 publications, 4.91%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 7, 4.29% American Institute of Physics (AIP) 7 publications, 4.29%
IOP Publishing	IOP Publishing, 5, 3.07% IOP Publishing 5 publications, 3.07%
Pleiades Publishing	Pleiades Publishing, 4, 2.45% Pleiades Publishing 4 publications, 2.45%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 1.84% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 1.84%
Chinese Physical Society	Chinese Physical Society, 3, 1.84% Chinese Physical Society 3 publications, 1.84%
Japan Society of Applied Physics	Japan Society of Applied Physics, 2, 1.23% Japan Society of Applied Physics 2 publications, 1.23%
American Vacuum Society	American Vacuum Society, 1, 0.61% American Vacuum Society 1 publication, 0.61%
Walter de Gruyter	Walter de Gruyter, 1, 0.61% Walter de Gruyter 1 publication, 0.61%
American Physical Society (APS)	American Physical Society (APS), 1, 0.61% American Physical Society (APS) 1 publication, 0.61%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.61% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.61%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.61% Research Square Platform LLC 1 publication, 0.61%
	10 20 30 40 50 60 70 80

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Yuan G. et al. Two Mechanisms Determine Quantum Dot Blinking. // ACS Nano. 2018. Vol. 12. No. 4. pp. 3397-3405.

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Yuan G., Gómez D. E., Kirkwood N., Boldt K., Mulvaney P. Two Mechanisms Determine Quantum Dot Blinking. // ACS Nano. 2018. Vol. 12. No. 4. pp. 3397-3405.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acsnano.7b09052

UR - https://doi.org/10.1021/acsnano.7b09052

TI - Two Mechanisms Determine Quantum Dot Blinking.

T2 - ACS Nano

AU - Yuan, Gangcheng

AU - Gómez, Daniel E.

AU - Boldt, Klaus

AU - Mulvaney, Paul

AU - Kirkwood, Nicholas

PY - 2018

DA - 2018/03/26 00:00:00

PB - American Chemical Society (ACS)

SP - 3397-3405

IS - 4

VL - 12

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

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BibTex Copy

@article{2018_Yuan,

author = {Gangcheng Yuan and Daniel E. Gómez and Klaus Boldt and Paul Mulvaney and Nicholas Kirkwood},

title = {Two Mechanisms Determine Quantum Dot Blinking.},

journal = {ACS Nano},

year = {2018},

volume = {12},

publisher = {American Chemical Society (ACS)},

month = {mar},

url = {https://doi.org/10.1021/acsnano.7b09052},

number = {4},

pages = {3397--3405},

doi = {10.1021/acsnano.7b09052}

}

MLA

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MLA Copy

Yuan, Gangcheng, et al. “Two Mechanisms Determine Quantum Dot Blinking..” ACS Nano, vol. 12, no. 4, Mar. 2018, pp. 3397-3405. https://doi.org/10.1021/acsnano.7b09052.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)