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volume 6 issue 35 pages 22740-22751

Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent

Vadim Filatov 1
Vadim E Filatov 1
Juliana Kuznetsova 1
Lada Petrovskaya 1
Dmitry Yuzabchuk 1
Victor A. Tafeenko 1
Nikolay V. Zyk 1
Publication typeJournal Article
Publication date2021-08-26
scimago Q1
wos Q2
SJR0.773
CiteScore7.1
Impact factor4.3
ISSN24701343
General Chemistry
General Chemical Engineering
Abstract
A convenient and versatile one-pot method for synthesis of 1,3-bis-aryl spirooxindolo-β-lactams from isatin Schiff bases and substituted phenylacetic acids using ketene–imine cycloaddition reaction with TsCl for a ketene generation has been developed. The reaction procedure does not require absolute solvents and unstable starting reagents. The studied reactions lead to cis-diastereoselective β-lactam formation for all tested phenylacetic acids except 4-MeOC6H4CH2COOH. An increase of trans-diastereomers yields with increasing temperature and solvent polarity was demonstrated.
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Filatov V. et al. Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent // ACS Omega. 2021. Vol. 6. No. 35. pp. 22740-22751.
GOST all authors (up to 50) Copy
Filatov V., Filatov V. E., Kuznetsova J., Petrovskaya L., Yuzabchuk D., Тафеенко В. А., Tafeenko V. A., Zyk N. V., Beloglazkina E. K. Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent // ACS Omega. 2021. Vol. 6. No. 35. pp. 22740-22751.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acsomega.1c03063
UR - https://pubs.acs.org/doi/10.1021/acsomega.1c03063
TI - Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent
T2 - ACS Omega
AU - Filatov, Vadim
AU - Filatov, Vadim E
AU - Kuznetsova, Juliana
AU - Petrovskaya, Lada
AU - Yuzabchuk, Dmitry
AU - Тафеенко, В. А.
AU - Tafeenko, Victor A.
AU - Zyk, Nikolay V.
AU - Beloglazkina, Elena K.
PY - 2021
DA - 2021/08/26
PB - American Chemical Society (ACS)
SP - 22740-22751
IS - 35
VL - 6
PMID - 34514245
SN - 2470-1343
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2021_Filatov,
author = {Vadim Filatov and Vadim E Filatov and Juliana Kuznetsova and Lada Petrovskaya and Dmitry Yuzabchuk and В. А. Тафеенко and Victor A. Tafeenko and Nikolay V. Zyk and Elena K. Beloglazkina},
title = {Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent},
journal = {ACS Omega},
year = {2021},
volume = {6},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://pubs.acs.org/doi/10.1021/acsomega.1c03063},
number = {35},
pages = {22740--22751},
doi = {10.1021/acsomega.1c03063}
}
MLA
Cite this
MLA Copy
Filatov, Vadim, et al. “Cis-Diastereoselective Synthesis of Spirooxindolo-β-Lactams by Staudinger Cycloaddition with TsCl as Activating Co-reagent.” ACS Omega, vol. 6, no. 35, Aug. 2021, pp. 22740-22751. https://pubs.acs.org/doi/10.1021/acsomega.1c03063.