Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System
Li Li
1, 2
,
Ersha Fan
1
,
Yibiao Guan
3
,
Xiaoxiao Zhang
1
,
Qing Xue
1
,
Wei Lei
1
,
Feng Wu
1, 2
,
Renjie Chen
1, 2
2
Collaborative Innovation Center of Electric Vehicles in Beijing, No. 5 South Zhongguancun Street, Beijing 100081, China
|
3
State Key Laboratory of Operation and Control of Renewable Energy & Storage Systems, China Electric Power Research Institute, Haidian District, Beijing 100192, China
|
Publication type: Journal Article
Publication date: 2017-05-11
scimago Q1
wos Q1
SJR: 1.623
CiteScore: 12.5
Impact factor: 7.3
ISSN: 21680485
General Chemistry
General Chemical Engineering
Environmental Chemistry
Renewable Energy, Sustainability and the Environment
Abstract
An environmentally friendly leaching process for recycling valuable metals from spent lithium-ion batteries is developed. A sol–gel method is utilized to resynthesize LiNi1/3Co1/3Mn1/3O2 from the leachate. Lactic acid is chosen as a leaching and chelating agent. The leaching efficiency is investigated by determining the contents of metal elements such as Li, Ni, Co, and Mn in the leachate using inductively coupled plasma optical emission spectroscopy. The spent cathode materials for the pretreatment process and the regenerated and freshly synthesized materials are examined using X-ray diffraction and scanning electronic microscopy. The results show that the leaching efficiencies of Li, Ni, Co, and Mn reached 97.7, 98.2, 98.9, and 98.4%, respectively. The optimum conditions are lactic acid concentration of 1.5 mol L–1, solid/liquid ratio of 20 g L–1, leaching temperature of 70 °C, H2O2 content of 0.5 vol %, and reaction time of 20 min. The leaching kinetics of cathode scrap in lactic acid fit well to the A...
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385
Total citations:
385
Citations from 2024:
110
(28%)
Cite this
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MLA
Cite this
GOST
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Li L. et al. Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System // ACS Sustainable Chemistry and Engineering. 2017. Vol. 5. No. 6. pp. 5224-5233.
GOST all authors (up to 50)
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Li L., Fan E., Guan Y., Zhang X., Xue Q., Lei W., Wu F., Chen R. Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System // ACS Sustainable Chemistry and Engineering. 2017. Vol. 5. No. 6. pp. 5224-5233.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acssuschemeng.7b00571
UR - https://doi.org/10.1021/acssuschemeng.7b00571
TI - Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System
T2 - ACS Sustainable Chemistry and Engineering
AU - Li, Li
AU - Fan, Ersha
AU - Guan, Yibiao
AU - Zhang, Xiaoxiao
AU - Xue, Qing
AU - Lei, Wei
AU - Wu, Feng
AU - Chen, Renjie
PY - 2017
DA - 2017/05/11
PB - American Chemical Society (ACS)
SP - 5224-5233
IS - 6
VL - 5
SN - 2168-0485
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Li,
author = {Li Li and Ersha Fan and Yibiao Guan and Xiaoxiao Zhang and Qing Xue and Wei Lei and Feng Wu and Renjie Chen},
title = {Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System},
journal = {ACS Sustainable Chemistry and Engineering},
year = {2017},
volume = {5},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acssuschemeng.7b00571},
number = {6},
pages = {5224--5233},
doi = {10.1021/acssuschemeng.7b00571}
}
Cite this
MLA
Copy
Li, Li, et al. “Sustainable Recovery of Cathode Materials from Spent Lithium-Ion Batteries Using Lactic Acid Leaching System.” ACS Sustainable Chemistry and Engineering, vol. 5, no. 6, May. 2017, pp. 5224-5233. https://doi.org/10.1021/acssuschemeng.7b00571.
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