Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex
Michael S Lowry
1
,
Jonas I. Goldsmith
1
,
Jason D. Slinker
1
,
Richard Rohl
1
,
Robert R. Pascal
1
,
Publication type: Journal Article
Publication date: 2005-10-13
scimago Q1
wos Q1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
We report the electronic structure and diverse applications of a highly luminescent ionic transition metal complex, [Ir(dF(CF3)ppy)2(dtbbpy)](PF6) (where dF(CF3)ppy = 2-(2,4-difluorophenyl)-5-trifluoromethylpyridine and dtbbpy = 4,4‘-di-tert-butyl-2,2‘-dipyridyl). The large HOMO−LUMO gap (ΔE = 3.06 V) enabled high-energy electroluminescence from the complex. Single-layer devices were fabricated and found to emit blue-green light (500 nm). The strong reducing strength of the excited state (E*ox = 1.21 V) enabled effective catalysis of the photoinduced reduction of H2O to H2. It was found that the relative quantum yield of hydrogen was over an order of magnitude improved from the standard photosensitizer Ru(dmphen)32+ (dmphen = 4,7-dimethyl-1,10-phenanthroline).
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857
Total citations:
857
Citations from 2024:
115
(13.42%)
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Lowry M. S. et al. Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex // Chemistry of Materials. 2005. Vol. 17. No. 23. pp. 5712-5719.
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Lowry M. S., Goldsmith J. I., Slinker J. D., Rohl R., Pascal R. R., Malliaras G. G., Bernhard S. Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex // Chemistry of Materials. 2005. Vol. 17. No. 23. pp. 5712-5719.
Cite this
RIS
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TY - JOUR
DO - 10.1021/cm051312+
UR - https://doi.org/10.1021/cm051312
TI - Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex
T2 - Chemistry of Materials
AU - Lowry, Michael S
AU - Goldsmith, Jonas I.
AU - Slinker, Jason D.
AU - Rohl, Richard
AU - Pascal, Robert R.
AU - Malliaras, George G
AU - Bernhard, Stefan
PY - 2005
DA - 2005/10/13
PB - American Chemical Society (ACS)
SP - 5712-5719
IS - 23
VL - 17
SN - 0897-4756
SN - 1520-5002
ER -
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BibTex (up to 50 authors)
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@article{2005_Lowry,
author = {Michael S Lowry and Jonas I. Goldsmith and Jason D. Slinker and Richard Rohl and Robert R. Pascal and George G Malliaras and Stefan Bernhard},
title = {Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex},
journal = {Chemistry of Materials},
year = {2005},
volume = {17},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/cm051312 },
number = {23},
pages = {5712--5719},
doi = {10.1021/cm051312+}
}
Cite this
MLA
Copy
Lowry, Michael S., et al. “Single-Layer Electroluminescent Devices and Photoinduced Hydrogen Production from an Ionic Iridium(III) Complex.” Chemistry of Materials, vol. 17, no. 23, Oct. 2005, pp. 5712-5719. https://doi.org/10.1021/cm051312 .