Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes
Тип публикации: Journal Article
Дата публикации: 2010-12-23
scimago Q1
wos Q1
БС1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Краткое описание
We demonstrate for the first time a possibility to vary the anion content in perovskites over a wide range through a long-range-ordered arrangement of crystallographic shear (CS) planes. Anion-deficient perovskites (Pb,Bi)1−xFe1+xO3−y with incommensurately modulated structures were prepared as single phases in the compositional range from Pb0.857Bi0.094Fe1.049O2.572 to Pb0.409Bi0.567Fe1.025O2.796. Using a combination of electron diffraction and high-resolution scanning transmission electron microscopy, we constructed a superspace model describing a periodic arrangement of the CS planes. The model was verified by refinement of the Pb0.64Bi0.32Fe1.04O2.675 crystal structure from neutron powder diffraction data ((3 + 1)D S.G. X2/m(α0γ), X = [1/2,1/2,1/2,1/2], a = 3.9082(1) A, b = 3.90333(8) A, c = 4.0900(1) A, β = 91.936(2)°, q = 0.05013(4)a* + 0.09170(3)c* at T = 700 K, RP = 0.036, RwP = 0.048). The (Pb,Bi)1−xFe1+xO3−y structures consist of perovskite blocks separated by CS planes confined to nearly the (50...
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Abakumov A. M. et al. Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes // Chemistry of Materials. 2010. Vol. 23. No. 2. pp. 255-265.
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Abakumov A. M., Batuk D., Hadermann J., Rozova M. G., Sheptyakov D., Sheptyakov D. V., Tsirlin A. A., Tsirlin A. A., Niermann D., Waschkowski F., Hemberger J., Hemberger J., Van Tendeloo G., Antipov E. V. Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes // Chemistry of Materials. 2010. Vol. 23. No. 2. pp. 255-265.
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TY - JOUR
DO - 10.1021/cm102907h
UR - https://pubs.acs.org/doi/10.1021/cm102907h
TI - Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes
T2 - Chemistry of Materials
AU - Abakumov, Artem M.
AU - Batuk, Dmitry
AU - Hadermann, Joke
AU - Rozova, Marina G
AU - Sheptyakov, Denis
AU - Sheptyakov, Denis V
AU - Tsirlin, A. A.
AU - Tsirlin, Alexander A.
AU - Niermann, Daniel
AU - Waschkowski, Florian
AU - Hemberger, J.
AU - Hemberger, Joachim
AU - Van Tendeloo, Gustaaf
AU - Antipov, Evgeny V.
PY - 2010
DA - 2010/12/23
PB - American Chemical Society (ACS)
SP - 255-265
IS - 2
VL - 23
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2010_Abakumov,
author = {Artem M. Abakumov and Dmitry Batuk and Joke Hadermann and Marina G Rozova and Denis Sheptyakov and Denis V Sheptyakov and A. A. Tsirlin and Alexander A. Tsirlin and Daniel Niermann and Florian Waschkowski and J. Hemberger and Joachim Hemberger and Gustaaf Van Tendeloo and Evgeny V. Antipov},
title = {Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes},
journal = {Chemistry of Materials},
year = {2010},
volume = {23},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://pubs.acs.org/doi/10.1021/cm102907h},
number = {2},
pages = {255--265},
doi = {10.1021/cm102907h}
}
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MLA
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Abakumov, Artem M., et al. “Antiferroelectric (Pb,Bi)1-xFe1+xO3-y perovskites modulated by crystallographic shear planes.” Chemistry of Materials, vol. 23, no. 2, Dec. 2010, pp. 255-265. https://pubs.acs.org/doi/10.1021/cm102907h.