MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties
Silvia Colella
1
,
P. Fedeli
3
,
Andrea Listorti
1, 4
,
Francesco Gazza
3, 5
,
F. Orlandi
3, 6
,
Patrizia Ferro
3
,
Tullo Besagni
3
,
Aurora Rizzo
1
,
G. Calestani
3, 6
,
Giuseppe Gigli
1, 4, 7
,
Roberto Mosca
3
2
Computational
Laboratory for Hybrid/Organic Photovoltaics (CLHYO), CNR-ISTM, Via Elce di Sotto 8, I-06123 Perugia, Italy
|
3
IMEM-CNR, Parco Area delle Scienze 37a, I-43124 Parma, Italy
|
5
Publication type: Journal Article
Publication date: 2013-11-11
scimago Q1
wos Q1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Hybrid halide perovskites represent one of the most promising solutions toward the fabrication of all solid nanostructured solar cells, with improved efficiency and long-term stability. This article aims at investigating the structural properties of iodide/chloride mixed-halide perovskites and correlating them with their photovoltaic performances. We found out that, independent of the components ratio in the precursor solution, Cl incorporation in an iodide-based structure, is possible only at relatively low concentration levels (below 3–4%). However, even if the material band gap remains substantially unchanged, the Cl doping dramatically improves the charge transport within the perovskite layer, explaining the outstanding performances of meso-superstructured solar cells based on this material.
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GOST
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Colella S. et al. MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties // Chemistry of Materials. 2013. Vol. 25. No. 22. pp. 4613-4618.
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Colella S., Edoardo Mosconi E., Fedeli P., Listorti A., Gazza F., Orlandi F., Ferro P., Besagni T., Rizzo A., Calestani G., Gigli G., De Angelis F., Mosca R. MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties // Chemistry of Materials. 2013. Vol. 25. No. 22. pp. 4613-4618.
Cite this
RIS
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TY - JOUR
DO - 10.1021/cm402919x
UR - https://doi.org/10.1021/cm402919x
TI - MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties
T2 - Chemistry of Materials
AU - Colella, Silvia
AU - Edoardo Mosconi, Edoardo
AU - Fedeli, P.
AU - Listorti, Andrea
AU - Gazza, Francesco
AU - Orlandi, F.
AU - Ferro, Patrizia
AU - Besagni, Tullo
AU - Rizzo, Aurora
AU - Calestani, G.
AU - Gigli, Giuseppe
AU - De Angelis, Filippo
AU - Mosca, Roberto
PY - 2013
DA - 2013/11/11
PB - American Chemical Society (ACS)
SP - 4613-4618
IS - 22
VL - 25
SN - 0897-4756
SN - 1520-5002
ER -
Cite this
BibTex (up to 50 authors)
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@article{2013_Colella,
author = {Silvia Colella and Edoardo Edoardo Mosconi and P. Fedeli and Andrea Listorti and Francesco Gazza and F. Orlandi and Patrizia Ferro and Tullo Besagni and Aurora Rizzo and G. Calestani and Giuseppe Gigli and Filippo De Angelis and Roberto Mosca},
title = {MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties},
journal = {Chemistry of Materials},
year = {2013},
volume = {25},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/cm402919x},
number = {22},
pages = {4613--4618},
doi = {10.1021/cm402919x}
}
Cite this
MLA
Copy
Colella, Silvia, et al. “MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties.” Chemistry of Materials, vol. 25, no. 22, Nov. 2013, pp. 4613-4618. https://doi.org/10.1021/cm402919x.