Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid
Lingyan Zhu
1
,
Fei Tong
1
,
Christopher Salinas
2
,
Muhanna K Al Muhanna
3
,
Fook S. Tham
1
,
David Kisailus
2, 4
,
Christopher J. Bardeen
1
Publication type: Journal Article
Publication date: 2014-10-07
scimago Q1
wos Q1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Four fluorinated derivatives of 9-anthracene carboxylic acid (9AC), a molecule that shows a reversible photomechanical response in its crystal form, have been synthesized and characterized. The spectroscopic properties and crystal structures of 4-fluoro-9-anthracene carboxylic acid (4F-9AC), 2-fluoro-9-anthracene carboxylic acid (2F-9AC), 10-fluoro-9-anthracene carboxylic acid (10F-9AC), and 2,6-difluoro-9-anthracene carboxylic acid (2,6DF-9AC) are all very similar to those of 9AC. However, their photomechanical properties vary widely. 405 nm light was used to induce [4 + 4] photodimerization and a mechanical response in crystalline microneedles and ribbons. Both the photodimer dissociation rate and the mechanical recovery varied by more than an order of magnitude, with 4F-9AC exhibiting the most rapid recovery time, on the order of 30 s. Nanoindentation measurements show that this crystal has a slightly reduced elastic modulus and a significantly reduced hardness, making it less brittle than the 9AC crys...
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76
Total citations:
76
Citations from 2024:
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(17.1%)
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GOST
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Zhu L. et al. Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid // Chemistry of Materials. 2014. Vol. 26. No. 20. pp. 6007-6015.
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Zhu L., Tong F., Salinas C., Al Muhanna M. K., Tham F. S., Kisailus D., Al-Kaysi R. O., Bardeen C. J. Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid // Chemistry of Materials. 2014. Vol. 26. No. 20. pp. 6007-6015.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/cm502866e
UR - https://doi.org/10.1021/cm502866e
TI - Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid
T2 - Chemistry of Materials
AU - Zhu, Lingyan
AU - Tong, Fei
AU - Salinas, Christopher
AU - Al Muhanna, Muhanna K
AU - Tham, Fook S.
AU - Kisailus, David
AU - Al-Kaysi, Rabih O.
AU - Bardeen, Christopher J.
PY - 2014
DA - 2014/10/07
PB - American Chemical Society (ACS)
SP - 6007-6015
IS - 20
VL - 26
SN - 0897-4756
SN - 1520-5002
ER -
Cite this
BibTex (up to 50 authors)
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@article{2014_Zhu,
author = {Lingyan Zhu and Fei Tong and Christopher Salinas and Muhanna K Al Muhanna and Fook S. Tham and David Kisailus and Rabih O. Al-Kaysi and Christopher J. Bardeen},
title = {Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid},
journal = {Chemistry of Materials},
year = {2014},
volume = {26},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/cm502866e},
number = {20},
pages = {6007--6015},
doi = {10.1021/cm502866e}
}
Cite this
MLA
Copy
Zhu, Lingyan, et al. “Improved Solid-State Photomechanical Materials by Fluorine Substitution of 9-Anthracene Carboxylic Acid.” Chemistry of Materials, vol. 26, no. 20, Oct. 2014, pp. 6007-6015. https://doi.org/10.1021/cm502866e.