Chemistry of Materials, volume 20, issue 1, pages 110-117
Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light
1
Department of Chemical System Engineering, School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-Ku, Tokyo 113-8656, Japan
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Publication type: Journal Article
Publication date: 2007-12-06
Journal:
Chemistry of Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 8.6
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Nanoporous CdS nanostructures, including nanosheets and hollow nanorods, have been prepared by a two-step aqueous route, which consists of a first precipitation of nanoporous Cd(OH)2 intermediates and a subsequent S2−/OH− ion-exchange conversion of the obtained Cd(OH)2 used as template either to nanoporous CdS nanosheets with sizes up to 60 nm and an average thickness of about 9 nm or to CdS hollow nanorods with lengths up to 30 nm and outer diameters in the range 7–14 nm. The obtained CdS nanostructures containing nanopores with diameters of ∼3 nm exhibit a very large BET surface area of about 112.8 m2 g−1. A very high hydrogen yield of about 4.1 mmol h−1 under visible light irradiation (λ ≥ 420 nm), corresponding to the highest apparent quantum yield of about 60.34% measured at 420 nm so far reported, has been attained over the obtained nanoporous CdS nanostructures loaded with monodisperse 3–5 nm Pt nanocrystals, which is due to an efficient charge separation, a fast transport of the photogenerated car...
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Bao N. et al. Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light // Chemistry of Materials. 2007. Vol. 20. No. 1. pp. 110-117.
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Bao N., Shen L., Takata T., Domen K. Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light // Chemistry of Materials. 2007. Vol. 20. No. 1. pp. 110-117.
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TY - JOUR
DO - 10.1021/cm7029344
UR - https://doi.org/10.1021/cm7029344
TI - Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light
T2 - Chemistry of Materials
AU - Bao, Ningzhong
AU - Shen, Liming
AU - Takata, Tsuyoshi
AU - Domen, Kazunari
PY - 2007
DA - 2007/12/06 00:00:00
PB - American Chemical Society (ACS)
SP - 110-117
IS - 1
VL - 20
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2007_Bao,
author = {Ningzhong Bao and Liming Shen and Tsuyoshi Takata and Kazunari Domen},
title = {Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light},
journal = {Chemistry of Materials},
year = {2007},
volume = {20},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/cm7029344},
number = {1},
pages = {110--117},
doi = {10.1021/cm7029344}
}
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Bao, Ningzhong, et al. “Self-Templated Synthesis of Nanoporous CdS Nanostructures for Highly Efficient Photocatalytic Hydrogen Production under Visible Light.” Chemistry of Materials, vol. 20, no. 1, Dec. 2007, pp. 110-117. https://doi.org/10.1021/cm7029344.