Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds
Publication type: Journal Article
Publication date: 2012-01-05
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Abstract
The hydrogenation of phenylacetone to cyclohexylacetone, in which the aromatic ring is selectively reduced in preference to the carbonyl group, has been achieved with chemoselectivities exceeding 90%. The catalyst (precatalyst) used to achieve this transformation comprises PVP-stabilized Rh nanoparticles dispersed in water with some phosphine ligand additives. Phosphine ligands with different steric and electronic properties and polarities were investigated for this purpose, and several clear trends were observed, showing the potential of well-defined phosphine ligands as modifiers in nanocatalysis.
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81
Total citations:
81
Citations from 2025:
4
(4.94%)
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GOST
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Snelders D. J. M. et al. Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds // ACS Catalysis. 2012. Vol. 2. No. 2. pp. 201-207.
GOST all authors (up to 50)
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Snelders D. J. M., Yan N., Gan W., Laurenczy G., Dyson P. J. Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds // ACS Catalysis. 2012. Vol. 2. No. 2. pp. 201-207.
Cite this
RIS
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TY - JOUR
DO - 10.1021/cs200575r
UR - https://doi.org/10.1021/cs200575r
TI - Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds
T2 - ACS Catalysis
AU - Snelders, Dennis J M
AU - Yan, Ning
AU - Gan, Weijia
AU - Laurenczy, Gabor
AU - Dyson, Paul J.
PY - 2012
DA - 2012/01/05
PB - American Chemical Society (ACS)
SP - 201-207
IS - 2
VL - 2
SN - 2155-5435
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2012_Snelders,
author = {Dennis J M Snelders and Ning Yan and Weijia Gan and Gabor Laurenczy and Paul J. Dyson},
title = {Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds},
journal = {ACS Catalysis},
year = {2012},
volume = {2},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/cs200575r},
number = {2},
pages = {201--207},
doi = {10.1021/cs200575r}
}
Cite this
MLA
Copy
Snelders, Dennis J. M., et al. “Tuning the Chemoselectivity of Rh Nanoparticle Catalysts by Site-Selective Poisoning with Phosphine Ligands: The Hydrogenation of Functionalized Aromatic Compounds.” ACS Catalysis, vol. 2, no. 2, Jan. 2012, pp. 201-207. https://doi.org/10.1021/cs200575r.