Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates
2
Department of Chemistry, Bowdoin College, Brunswick, Maine 04011, United States
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Publication type: Journal Article
Publication date: 2014-06-30
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
24978813
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
A series of thienyl pyrazole proligands and gold(I) thienyl pyrazolate cyclic trinuclear complexes (CTCs) have been synthesized. The relationship between the structure and emission properties of bridging thienyl pyrazolates within gold(I) cyclic trinuclear complexes suggests that the nature of dual emission is sensitive to ligand conjugation length. Density functional theory has been used to support the assignment of metal-sensitized, ligand-localized phosphorescence from monothienyl complexes, while low-lying, ligand-localized LUMOs present in bithienyl systems prohibit metal-sensitized phosphorescence. Soluble n-hexyl derivatives have been synthesized to explore the electrochemical properties of gold(I) thienyl pyrazolates CTCs, and conductive electropolymerized thin films were realized.
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Total citations:
27
Citations from 2025:
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(3.7%)
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Earl L. D., Nagle J. K., Wolf M. O. Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates // Inorganic Chemistry. 2014. Vol. 53. No. 14. pp. 7106-7117.
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Earl L. D., Nagle J. K., Wolf M. O. Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates // Inorganic Chemistry. 2014. Vol. 53. No. 14. pp. 7106-7117.
Cite this
RIS
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TY - JOUR
DO - 10.1021/ic4031365
UR - https://doi.org/10.1021/ic4031365
TI - Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates
T2 - Inorganic Chemistry
AU - Earl, Lyndsey D
AU - Nagle, Jeffrey K.
AU - Wolf, M O
PY - 2014
DA - 2014/06/30
PB - American Chemical Society (ACS)
SP - 7106-7117
IS - 14
VL - 53
PMID - 24978813
SN - 0020-1669
SN - 1520-510X
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2014_Earl,
author = {Lyndsey D Earl and Jeffrey K. Nagle and M O Wolf},
title = {Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates},
journal = {Inorganic Chemistry},
year = {2014},
volume = {53},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/ic4031365},
number = {14},
pages = {7106--7117},
doi = {10.1021/ic4031365}
}
Cite this
MLA
Copy
Earl, Lyndsey D., et al. “Tuning the Extended Structure and Electronic Properties of Gold(I) Thienyl Pyrazolates.” Inorganic Chemistry, vol. 53, no. 14, Jun. 2014, pp. 7106-7117. https://doi.org/10.1021/ic4031365.