Inorganic Chemistry

, том 53 , издание 18 , страницы 9463-9465

Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes

Тип публикации: Journal Article

Дата публикации: 2014-08-29

American Chemical Society (ACS)

Inorganic Chemistry

scimago Q1

wos Q1

БС1

SJR: 0.928

CiteScore: 7.6

Impact factor: 4.7

ISSN: 00201669, 1520510X

DOI: 10.1021/ic501901n

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PubMed ID: 25171221

Inorganic Chemistry

Physical and Theoretical Chemistry

Краткое описание

The addition of carbon dioxide to ((tBu)PNP)CoH [(tBu)PNP = 2,6-bis(di-tert-butylphosphinomethyl)pyridine] resulted in rapid insertion into the Co-H bond to form the corresponding κ(1)-formate complex, which has been structurally characterized. Treatment of ((tBu)PNP)CoH with PhSiH3 resulted in oxidative addition to form trans-((tBu)PNP)CoH2(SiH2Ph), which undergoes rapid exchange with excess free silane. With 0.5 mol % ((tBu)PNP)CoH, the catalytic hydrosilylation of CO2 with PhSiH3 to a mixture of oligomers containing silyl formate, bis(silyl)acetyl, and silyl ether subunits has been observed.

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ГОСТ |

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Scheuermann M. L. et al. Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes // Inorganic Chemistry. 2014. Vol. 53. No. 18. pp. 9463-9465.

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Scheuermann M. L., Semproni S. P., Pappas I., Chirik P. J. Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes // Inorganic Chemistry. 2014. Vol. 53. No. 18. pp. 9463-9465.

RIS |

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TY - JOUR

DO - 10.1021/ic501901n

UR - https://doi.org/10.1021/ic501901n

TI - Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes

T2 - Inorganic Chemistry

AU - Scheuermann, Margaret L

AU - Semproni, Scott P

AU - Pappas, Iraklis

AU - Chirik, Paul J.

PY - 2014

DA - 2014/08/29

PB - American Chemical Society (ACS)

SP - 9463-9465

IS - 18

VL - 53

PMID - 25171221

SN - 0020-1669

SN - 1520-510X

ER -

BibTex |

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@article{2014_Scheuermann,

author = {Margaret L Scheuermann and Scott P Semproni and Iraklis Pappas and Paul J. Chirik},

title = {Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes},

journal = {Inorganic Chemistry},

year = {2014},

volume = {53},

publisher = {American Chemical Society (ACS)},

month = {aug},

url = {https://doi.org/10.1021/ic501901n},

number = {18},

pages = {9463--9465},

doi = {10.1021/ic501901n}

}

MLA

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MLA Скопировать

Scheuermann, Margaret L., et al. “Carbon Dioxide Hydrosilylation Promoted by Cobalt Pincer Complexes.” Inorganic Chemistry, vol. 53, no. 18, Aug. 2014, pp. 9463-9465. https://doi.org/10.1021/ic501901n.

Издатель

American Chemical Society (ACS)

Журнал

Inorganic Chemistry

scimago Q1

wos Q1

БС1

SJR

0.928

CiteScore

7.6

Impact factor

4.7

ISSN

00201669 (Print)

1520510X (Electronic)