Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes
Тип публикации: Journal Article
Дата публикации: 2015-03-23
scimago Q1
wos Q1
БС1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
25797500
Inorganic Chemistry
Physical and Theoretical Chemistry
Краткое описание
The three new complexes Tp(Py)Ln(CH3CO2)2(H2O) (Ln = Eu (1), Gd(2), or Tb (3)) were prepared and characterized crystallographically. In the crystal lattices of these complexes, separate molecules are connected in infinite chains by π-stacking interactions. Complexes 1 and 3 display intense photoluminescence and triboluminescence (red and green respectively), while compound 3 exhibits electroluminescence commencing at 9 V in an ITO/PVK/3/Al device (ITO = indium-tin oxide, PVK = poly(N-vinylcarbazole)). A series of Eu/Tb-doped Gd compounds was prepared by cocrystallization from mixtures of 1 and 2 or 2 and 3, respectively. It was shown that π-stacking interactions are involved in increasing the efficiency of energy transfer from the gadolinium complex to emitting [Tp(Py)Eu](2+) or [Tp(Py)Tb](2+) centers, and this energy transfer occurs through hundreds of molecules, resembling the process of energy harvesting in chloroplast stacks.
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Mikhalyova E. A. et al. Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes // Inorganic Chemistry. 2015. Vol. 54. No. 7. pp. 3125-3133.
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Mikhalyova E. A., Yakovenko A. V., Zeller M. W., Kiskin M. A., Kolomzarov Y. V., Eremenko I. L., Addison A. W., Pavlishchuk V. V. Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes // Inorganic Chemistry. 2015. Vol. 54. No. 7. pp. 3125-3133.
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TY - JOUR
DO - 10.1021/ic502120g
UR - https://doi.org/10.1021/ic502120g
TI - Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes
T2 - Inorganic Chemistry
AU - Mikhalyova, Elena A
AU - Yakovenko, Anastasiya V
AU - Zeller, Matthias W.
AU - Kiskin, Mikhail A.
AU - Kolomzarov, Yuriy V
AU - Eremenko, Igor L.
AU - Addison, Anthony W.
AU - Pavlishchuk, Vitaly V
PY - 2015
DA - 2015/03/23
PB - American Chemical Society (ACS)
SP - 3125-3133
IS - 7
VL - 54
PMID - 25797500
SN - 0020-1669
SN - 1520-510X
ER -
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@article{2015_Mikhalyova,
author = {Elena A Mikhalyova and Anastasiya V Yakovenko and Matthias W. Zeller and Mikhail A. Kiskin and Yuriy V Kolomzarov and Igor L. Eremenko and Anthony W. Addison and Vitaly V Pavlishchuk},
title = {Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes},
journal = {Inorganic Chemistry},
year = {2015},
volume = {54},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/ic502120g},
number = {7},
pages = {3125--3133},
doi = {10.1021/ic502120g}
}
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MLA
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Mikhalyova, Elena A., et al. “Manifestation of π–π Stacking Interactions in Luminescence Properties and Energy Transfer in Aromatically-Derived Tb, Eu and Gd Tris(pyrazolyl)borate Complexes.” Inorganic Chemistry, vol. 54, no. 7, Mar. 2015, pp. 3125-3133. https://doi.org/10.1021/ic502120g.