Journal of the American Chemical Society, volume 112, issue 4, pages 1327-1332
Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media
Publication type: Journal Article
Publication date: 1990-02-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 15
ISSN: 00027863, 15205126
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Composite semiconductor crystallites involving CdSe grown on an ZnS seed, and vice versa, have been synthesized and capped with organic ligands in inverse micelle solutions. These composite particles, as well as capped seed crystallites of CdSe and ZnS, are isolated, purified, and characterized for relative atomic composition, structure, and electronic properties. The Debye X-ray scattering equation, when solved for these layered particles, shows that powder X-ray scattering is insensitive to a small foreign inclusion. A simple theoretical model for the LUMO and HOMO of layered crystallites shows that a small (< 15-{angstrom} diameter) interior foreign seed causes only small shifts of the lowest excited state, to either higher or lower energies. The capped CdSe seed and the capped CdSe portion of the layered particle grown on a ZnSe seed undergo low-temperature (169{degree}C) annealing to give near-single-crystal X-ray scattering. However, CdSe annealing is blocked by a surface ZnS layer which is ca. 4 {angstrom} thick. While growth to make composite particles does occur, neither particle shows evidence for epitaxial growth.
Top-30
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Citations by publishers
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Elsevier
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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KORTAN A. R. et al. Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media // Journal of the American Chemical Society. 1990. Vol. 112. No. 4. pp. 1327-1332.
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KORTAN A. R., Hull R., Opila R., Bawendi M. G., Steigerwald M., CARROLL P. J., Brus L. Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media // Journal of the American Chemical Society. 1990. Vol. 112. No. 4. pp. 1327-1332.
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TY - JOUR
DO - 10.1021/ja00160a005
UR - https://doi.org/10.1021/ja00160a005
TI - Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media
T2 - Journal of the American Chemical Society
AU - KORTAN, A. R.
AU - Hull, R.
AU - CARROLL, P J
AU - Opila, R.
AU - Bawendi, Moungi G.
AU - Steigerwald, Michael
AU - Brus, Louis
PY - 1990
DA - 1990/02/01 00:00:00
PB - American Chemical Society (ACS)
SP - 1327-1332
IS - 4
VL - 112
SN - 0002-7863
SN - 1520-5126
ER -
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@article{1990_KORTAN,
author = {A. R. KORTAN and R. Hull and P J CARROLL and R. Opila and Moungi G. Bawendi and Michael Steigerwald and Louis Brus},
title = {Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media},
journal = {Journal of the American Chemical Society},
year = {1990},
volume = {112},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/ja00160a005},
number = {4},
pages = {1327--1332},
doi = {10.1021/ja00160a005}
}
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KORTAN, A. R., et al. “Nucleation and Growth of CdSe on ZnS Quantum Crystallite Seeds and Vice Versa, in Inverse Micelle Media.” Journal of the American Chemical Society, vol. 112, no. 4, Feb. 1990, pp. 1327-1332. https://doi.org/10.1021/ja00160a005.