Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites.
Тип публикации: Journal Article
Дата публикации: 2005-01-15
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
15686370
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
This work reports on the capability of the O2-activated Cu-ZSM-5 and Cu-MOR zeolites to selectively convert methane into methanol at a temperature of 398 K. A strong correlation between (i) the activity and (ii) the intensity of the 22 700 cm-1 UV-vis band, assigned to the bis(mu-oxo)dicopper core, is found (i) as a function of the reaction temperature, (ii) as a function of the Cu loading of the zeolite, and (iii) in comparison to other Cu materials. These three lines of evidence firmly support the key role of the bis(mu-oxo)dicopper core in this selective, low-temperature hydroxylation of methane.
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Groothaert M. H. et al. Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites. // Journal of the American Chemical Society. 2005. Vol. 127. No. 5. pp. 1394-1395.
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Groothaert M. H., Smeets P. J., Sels B. F., Jacobs P. A., Schoonheydt R. A. Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites. // Journal of the American Chemical Society. 2005. Vol. 127. No. 5. pp. 1394-1395.
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TY - JOUR
DO - 10.1021/ja047158u
UR - https://doi.org/10.1021/ja047158u
TI - Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites.
T2 - Journal of the American Chemical Society
AU - Groothaert, Marijke H
AU - Smeets, Pieter J
AU - Sels, Bert F
AU - Jacobs, Pierre A.
AU - Schoonheydt, R. A.
PY - 2005
DA - 2005/01/15
PB - American Chemical Society (ACS)
SP - 1394-1395
IS - 5
VL - 127
PMID - 15686370
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2005_Groothaert,
author = {Marijke H Groothaert and Pieter J Smeets and Bert F Sels and Pierre A. Jacobs and R. A. Schoonheydt},
title = {Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites.},
journal = {Journal of the American Chemical Society},
year = {2005},
volume = {127},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/ja047158u},
number = {5},
pages = {1394--1395},
doi = {10.1021/ja047158u}
}
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MLA
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Groothaert, Marijke H., et al. “Selective oxidation of methane by the bis(mu-oxo)dicopper core stabilized on ZSM-5 and mordenite zeolites..” Journal of the American Chemical Society, vol. 127, no. 5, Jan. 2005, pp. 1394-1395. https://doi.org/10.1021/ja047158u.
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