Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells
Liwen Ji
1
,
Mumin Rao
2
,
Haimei Zheng
3
,
Liang Zhang
4
,
Yuanchang Li
5
,
Wenhui Duan
5
,
Jinghua Guo
4
,
Elton J. Cairns
2
,
Yuegang Zhang
1
Publication type: Journal Article
Publication date: 2011-11-01
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
22017295
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
The loss of sulfur cathode material as a result of polysulfide dissolution causes significant capacity fading in rechargeable lithium/sulfur cells. Here, we use a chemical approach to immobilize sulfur and lithium polysulfides via the reactive functional groups on graphene oxide. This approach enabled us to obtain a uniform and thin (around tens of nanometers) sulfur coating on graphene oxide sheets by a simple chemical reaction-deposition strategy and a subsequent low-temperature thermal treatment process. Strong interaction between graphene oxide and sulfur or polysulfides enabled us to demonstrate lithium/sulfur cells with a high reversible capacity of 950-1400 mA h g(-1), and stable cycling for more than 50 deep cycles at 0.1C (1C = 1675 mA g(-1)).
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Ji L. et al. Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells // Journal of the American Chemical Society. 2011. Vol. 133. No. 46. pp. 18522-18525.
GOST all authors (up to 50)
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Ji L., Rao M., Zheng H., Zhang L., Li Y., Duan W., Guo J., Cairns E. J., Zhang Y. Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells // Journal of the American Chemical Society. 2011. Vol. 133. No. 46. pp. 18522-18525.
Cite this
RIS
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TY - JOUR
DO - 10.1021/ja206955k
UR - https://doi.org/10.1021/ja206955k
TI - Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells
T2 - Journal of the American Chemical Society
AU - Ji, Liwen
AU - Rao, Mumin
AU - Zheng, Haimei
AU - Zhang, Liang
AU - Li, Yuanchang
AU - Duan, Wenhui
AU - Guo, Jinghua
AU - Cairns, Elton J.
AU - Zhang, Yuegang
PY - 2011
DA - 2011/11/01
PB - American Chemical Society (ACS)
SP - 18522-18525
IS - 46
VL - 133
PMID - 22017295
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2011_Ji,
author = {Liwen Ji and Mumin Rao and Haimei Zheng and Liang Zhang and Yuanchang Li and Wenhui Duan and Jinghua Guo and Elton J. Cairns and Yuegang Zhang},
title = {Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells},
journal = {Journal of the American Chemical Society},
year = {2011},
volume = {133},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/ja206955k},
number = {46},
pages = {18522--18525},
doi = {10.1021/ja206955k}
}
Cite this
MLA
Copy
Ji, Liwen, et al. “Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells.” Journal of the American Chemical Society, vol. 133, no. 46, Nov. 2011, pp. 18522-18525. https://doi.org/10.1021/ja206955k.