Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N
Тип публикации: Journal Article
Дата публикации: 2012-02-14
scimago Q1
wos Q1
БС1
SJR: 5.489
CiteScore: 24.4
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
22316385
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
We report a synergistic effect involving hydrogenation and nitridation cotreatment of TiO(2) nanowire (NW) arrays that improves the water photo-oxidation performance under visible light illumination. The visible light (>420 nm) photocurrent of the cotreated TiO(2) is 0.16 mA/cm(2) and accounts for 41% of the total photocurrent under simulated AM 1.5 G illumination. Electron paramagnetic resonance (EPR) spectroscopy reveals that the concentration of Ti(3+) species in the bulk of the TiO(2) following hydrogenation and nitridation cotreatment is significantly higher than that of the sample treated solely with ammonia. It is believed that the interaction between the N-dopant and Ti(3+) is the key to the extension of the active spectrum and the superior visible light water photo-oxidation activity of the hydrogenation and nitridation cotreated TiO(2) NW arrays.
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Hoang S. et al. Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N // Journal of the American Chemical Society. 2012. Vol. 134. No. 8. pp. 3659-3662.
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Hoang S., Berglund S. P., Hahn N. T., Bard A., Mullins C. B. Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N // Journal of the American Chemical Society. 2012. Vol. 134. No. 8. pp. 3659-3662.
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TY - JOUR
DO - 10.1021/ja211369s
UR - https://doi.org/10.1021/ja211369s
TI - Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N
T2 - Journal of the American Chemical Society
AU - Hoang, Son
AU - Berglund, Sean P
AU - Hahn, Nathan T
AU - Bard, Allen
AU - Mullins, C. Buddie
PY - 2012
DA - 2012/02/14
PB - American Chemical Society (ACS)
SP - 3659-3662
IS - 8
VL - 134
PMID - 22316385
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2012_Hoang,
author = {Son Hoang and Sean P Berglund and Nathan T Hahn and Allen Bard and C. Buddie Mullins},
title = {Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N},
journal = {Journal of the American Chemical Society},
year = {2012},
volume = {134},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/ja211369s},
number = {8},
pages = {3659--3662},
doi = {10.1021/ja211369s}
}
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Hoang, Son, et al. “Enhancing Visible Light Photo-oxidation of Water with TiO2 Nanowire Arrays via Cotreatment with H2 and NH3: Synergistic Effects between Ti3+ and N.” Journal of the American Chemical Society, vol. 134, no. 8, Feb. 2012, pp. 3659-3662. https://doi.org/10.1021/ja211369s.