A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation
Publication type: Journal Article
Publication date: 2013-04-02
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
23548055
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
The coupling of O-pivaloyl benzhydroxamic acids with donor/acceptor diazo compounds provides isoindolones in high yield. The reaction tolerates a broad range of benzhydroxamic acids and diazo compounds, including substituted 2,2,2-trifluorodiazoethanes. Mechanistic experiments suggested that C-H activation is turnover-limiting and irreversible and that insertion of the diazo compound favors electron-deficient substrates.
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481
Total citations:
481
Citations from 2025:
8
(1.67%)
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Hyster T., Ruhl K. E., Rovis T. A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation // Journal of the American Chemical Society. 2013. Vol. 135. No. 14. pp. 5364-5367.
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Hyster T., Ruhl K. E., Rovis T. A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation // Journal of the American Chemical Society. 2013. Vol. 135. No. 14. pp. 5364-5367.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ja402274g
UR - https://doi.org/10.1021/ja402274g
TI - A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation
T2 - Journal of the American Chemical Society
AU - Hyster, Todd
AU - Ruhl, Kyle E
AU - Rovis, Tomislav
PY - 2013
DA - 2013/04/02
PB - American Chemical Society (ACS)
SP - 5364-5367
IS - 14
VL - 135
PMID - 23548055
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2013_Hyster,
author = {Todd Hyster and Kyle E Ruhl and Tomislav Rovis},
title = {A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation},
journal = {Journal of the American Chemical Society},
year = {2013},
volume = {135},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/ja402274g},
number = {14},
pages = {5364--5367},
doi = {10.1021/ja402274g}
}
Cite this
MLA
Copy
Hyster, Todd, et al. “A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation.” Journal of the American Chemical Society, vol. 135, no. 14, Apr. 2013, pp. 5364-5367. https://doi.org/10.1021/ja402274g.