Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes
Тип публикации: Journal Article
Дата публикации: 2013-09-04
scimago Q1
wos Q1
БС1
SJR: 5.489
CiteScore: 24.4
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
23971827
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
The two-coordinate cationic Ni(I) bis-N-heterocyclic carbene complex [Ni(6-Mes)2]Br (1) [6-Mes =1,3-bis(2,4,6-trimethylphenyl)-3,4,5,6-tetrahydropyrimidin-2-ylidene] has been structurally characterized and displays a highly linear geometry with a C-Ni-C angle of 179.27(13)°. Density functional theory calculations revealed that the five occupied metal-based orbitals are split in an approximate 2:1:2 pattern. Significant magnetic anisotropy results from this orbital degeneracy, leading to single-ion magnet (SIM) behavior.
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Poulten R. C. et al. Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes // Journal of the American Chemical Society. 2013. Vol. 135. No. 37. pp. 13640-13643.
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Poulten R. C., Page M., Algarra A. G., Le Roy J. J., López I., Carter E., Llobet A., Macgregor S., Mahon M. F., Murphy D. B., Murugesu M., Whittlesey M. Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes // Journal of the American Chemical Society. 2013. Vol. 135. No. 37. pp. 13640-13643.
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TY - JOUR
DO - 10.1021/ja407004y
UR - https://doi.org/10.1021/ja407004y
TI - Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes
T2 - Journal of the American Chemical Society
AU - Poulten, Rebecca C
AU - Page, Michael J.
AU - Algarra, Andrés G.
AU - Le Roy, Jennifer J.
AU - López, Isidoro
AU - Carter, Emma
AU - Llobet, A.
AU - Macgregor, Stuart
AU - Mahon, Mary F.
AU - Murphy, Damien B.
AU - Murugesu, Muralee
AU - Whittlesey, Michael
PY - 2013
DA - 2013/09/04
PB - American Chemical Society (ACS)
SP - 13640-13643
IS - 37
VL - 135
PMID - 23971827
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2013_Poulten,
author = {Rebecca C Poulten and Michael J. Page and Andrés G. Algarra and Jennifer J. Le Roy and Isidoro López and Emma Carter and A. Llobet and Stuart Macgregor and Mary F. Mahon and Damien B. Murphy and Muralee Murugesu and Michael Whittlesey},
title = {Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes},
journal = {Journal of the American Chemical Society},
year = {2013},
volume = {135},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/ja407004y},
number = {37},
pages = {13640--13643},
doi = {10.1021/ja407004y}
}
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MLA
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Poulten, Rebecca C., et al. “Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes.” Journal of the American Chemical Society, vol. 135, no. 37, Sep. 2013, pp. 13640-13643. https://doi.org/10.1021/ja407004y.