Journal of the American Chemical Society, volume 136, issue 25, pages 8883-8886

Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100).

Ju Young Woo ¹

Jae-Hyeon Ko ²

Jung Hoon Song ¹

Kyungnam Kim ¹

Hyekyoung Choi ^{1, 3}

Y H Kim ²

Doh Jae Lee

So-Hee Jeong ^{1, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

Nanomechanical Systems Research Division, Korea Institute of Machinery and Materials (KIMM), Daejeon 305-343, Korea |

Center for Nanomaterials and Chemical Reactions, Institute for Basic Science (IBS), Daejeon 305-701, Korea |

Department of Nanomechatronics, Korea University of Science and Technology (UST), Daejeon 305-350, Korea |

Publication type: Journal Article

Publication date: 2014-06-17

American Chemical Society (ACS)

Journal: Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor: 15

ISSN: 00027863, 15205126

DOI: 10.1021/ja503957r

Copy DOI

General Chemistry

Catalysis

Biochemistry

Colloid and Surface Chemistry

Abstract

The fast degradation of lead selenide (PbSe) nanocrystal quantum dots (NQDs) in ambient conditions impedes widespread deployment of the highly excitonic, thus versatile, colloidal NQDs. Here we report a simple in situ post-synthetic halide salt treatment that results in size-independent air stability of PbSe NQDs without significantly altering their optoelectronic characteristics. From TEM, NMR, and XPS results and DFT calculations, we propose that the unprecedented size-independent air stability of the PbSe NQDs can be attributed to the successful passivation of under-coordinated PbSe(100) facets with atomically thin PbX2 (X = Cl, Br, I) adlayers. Conductive films made of halide-treated ultrastable PbSe NQDs exhibit markedly improved air stability and behave as an n-type channel in a field-effect transistor. Our simple in situ wet-chemical passivation scheme will enable broader utilization of PbSe NQDs in ambient conditions in many optoelectronic applications.

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International Journal of Molecular Sciences	International Journal of Molecular Sciences, 1, 0.59% International Journal of Molecular Sciences 1 publication, 0.59%
	2 4 6 8 10 12 14 16

Citations by publishers

	10 20 30 40 50 60
American Chemical Society (ACS)	American Chemical Society (ACS), 60, 35.29% American Chemical Society (ACS) 60 publications, 35.29%
Wiley	Wiley, 38, 22.35% Wiley 38 publications, 22.35%
Elsevier	Elsevier, 17, 10% Elsevier 17 publications, 10%
Springer Nature	Springer Nature, 16, 9.41% Springer Nature 16 publications, 9.41%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 1.18% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 1.18%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.59% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.59%
Japan Society of Applied Physics	Japan Society of Applied Physics, 1, 0.59% Japan Society of Applied Physics 1 publication, 0.59%
Pleiades Publishing	Pleiades Publishing, 1, 0.59% Pleiades Publishing 1 publication, 0.59%
Taylor & Francis	Taylor & Francis, 1, 0.59% Taylor & Francis 1 publication, 0.59%
Walter de Gruyter	Walter de Gruyter, 1, 0.59% Walter de Gruyter 1 publication, 0.59%
Optical Society of America	Optical Society of America, 1, 0.59% Optical Society of America 1 publication, 0.59%
Hindawi Limited	Hindawi Limited, 1, 0.59% Hindawi Limited 1 publication, 0.59%
Korean Ceramic Society	Korean Ceramic Society, 1, 0.59% Korean Ceramic Society 1 publication, 0.59%
Future Medicine	Future Medicine, 1, 0.59% Future Medicine 1 publication, 0.59%
	10 20 30 40 50 60

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Woo J. Y. et al. Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100). // Journal of the American Chemical Society. 2014. Vol. 136. No. 25. pp. 8883-8886.

GOST all authors (up to 50) Copy

Woo J. Y., Ko J., Song J. H., Kim K., Choi H., Kim Y. H., Lee D. J., Jeong S. Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100). // Journal of the American Chemical Society. 2014. Vol. 136. No. 25. pp. 8883-8886.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/ja503957r

UR - https://doi.org/10.1021/ja503957r

TI - Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100).

T2 - Journal of the American Chemical Society

AU - Woo, Ju Young

AU - Ko, Jae-Hyeon

AU - Song, Jung Hoon

AU - Kim, Kyungnam

AU - Choi, Hyekyoung

AU - Kim, Y H

AU - Lee, Doh Jae

AU - Jeong, So-Hee

PY - 2014

DA - 2014/06/17 00:00:00

PB - American Chemical Society (ACS)

SP - 8883-8886

IS - 25

VL - 136

SN - 0002-7863

SN - 1520-5126

ER -

BibTex |

Cite this

BibTex Copy

@article{2014_Woo,

author = {Ju Young Woo and Jae-Hyeon Ko and Jung Hoon Song and Kyungnam Kim and Hyekyoung Choi and Y H Kim and Doh Jae Lee and So-Hee Jeong},

title = {Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100).},

journal = {Journal of the American Chemical Society},

year = {2014},

volume = {136},

publisher = {American Chemical Society (ACS)},

month = {jun},

url = {https://doi.org/10.1021/ja503957r},

number = {25},

pages = {8883--8886},

doi = {10.1021/ja503957r}

}

MLA

Cite this

MLA Copy

Woo, Ju Young, et al. “Ultrastable PbSe nanocrystal quantum dots via in situ formation of atomically thin halide adlayers on PbSe(100)..” Journal of the American Chemical Society, vol. 136, no. 25, Jun. 2014, pp. 8883-8886. https://doi.org/10.1021/ja503957r.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor

ISSN

00027863 (Print)
15205126 (Electronic)