Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications.
Publication type: Journal Article
Publication date: 2014-08-12
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
25075458
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Using time-resolved photoluminescence and transient absorption measurements at room temperature, we report excitation-intensity-dependent photocarrier recombination processes in thin films made from the organo-metal halide perovskite semiconductor CH3NH3PbI3 for solar-cell applications. The photocarrier dynamics are well described by a simple rate equation including single-carrier trapping and electron-hole radiative recombination. This result provides clear evidence that the free-carrier model is better than the exciton model for interpreting the optical properties of CH3NH3PbI3. The observed large two-carrier recombination rate suggests the promising potential of perovskite semiconductors for optoelectronic device applications. Our findings provide the information about the dynamical behaviors of photoexcited carriers that is needed for developing high-efficiency perovskite solar cells.
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Total citations:
756
Citations from 2025:
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(5.16%)
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Yamada Y. et al. Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications. // Journal of the American Chemical Society. 2014. Vol. 136. No. 33. pp. 11610-11613.
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Yamada Y., NAKAMURA T., Endo M., Wakamiya A., Kanemitsu Y. Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications. // Journal of the American Chemical Society. 2014. Vol. 136. No. 33. pp. 11610-11613.
Cite this
RIS
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TY - JOUR
DO - 10.1021/ja506624n
UR - https://doi.org/10.1021/ja506624n
TI - Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications.
T2 - Journal of the American Chemical Society
AU - Yamada, Yasuhiro
AU - NAKAMURA, Toru
AU - Endo, Masaru
AU - Wakamiya, Atsushi
AU - Kanemitsu, Yoshihiko
PY - 2014
DA - 2014/08/12
PB - American Chemical Society (ACS)
SP - 11610-11613
IS - 33
VL - 136
PMID - 25075458
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (up to 50 authors)
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@article{2014_Yamada,
author = {Yasuhiro Yamada and Toru NAKAMURA and Masaru Endo and Atsushi Wakamiya and Yoshihiko Kanemitsu},
title = {Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications.},
journal = {Journal of the American Chemical Society},
year = {2014},
volume = {136},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/ja506624n},
number = {33},
pages = {11610--11613},
doi = {10.1021/ja506624n}
}
Cite this
MLA
Copy
Yamada, Yasuhiro, et al. “Photocarrier recombination dynamics in perovskite CH3NH3PbI3 for solar cell applications..” Journal of the American Chemical Society, vol. 136, no. 33, Aug. 2014, pp. 11610-11613. https://doi.org/10.1021/ja506624n.