Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions
Тип публикации: Journal Article
Дата публикации: 2008-04-01
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22
Impact factor: 16.6
ISSN: 00027863, 15205126
PubMed ID:
18393504
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
A new family of phosphinthiourea catalysts was developed for the highly enantioselective synthesis of 2-aryl-2,5-hydropyrroles via a [3 + 2] cycloaddition of an electron-deficient allene with aryl and heteroaryl diphenylphosphinoylimines. The presence of both H2O and Et3N as additives was found to be important for achieving optimal rates. Dual activation of both nucleophile and electrophile by the bifunctional catalyst is invoked to account for the observed high reactivity and enantioselectivity.
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ГОСТ
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Fang Y. Q., Jacobsen E. Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions // Journal of the American Chemical Society. 2008. Vol. 130. No. 17. pp. 5660-5661.
ГОСТ со всеми авторами (до 50)
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Fang Y. Q., Jacobsen E. Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions // Journal of the American Chemical Society. 2008. Vol. 130. No. 17. pp. 5660-5661.
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TY - JOUR
DO - 10.1021/ja801344w
UR - https://doi.org/10.1021/ja801344w
TI - Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions
T2 - Journal of the American Chemical Society
AU - Fang, Yuan Qing
AU - Jacobsen, Eric
PY - 2008
DA - 2008/04/01
PB - American Chemical Society (ACS)
SP - 5660-5661
IS - 17
VL - 130
PMID - 18393504
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (до 50 авторов)
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@article{2008_Fang,
author = {Yuan Qing Fang and Eric Jacobsen},
title = {Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions},
journal = {Journal of the American Chemical Society},
year = {2008},
volume = {130},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/ja801344w},
number = {17},
pages = {5660--5661},
doi = {10.1021/ja801344w}
}
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MLA
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Fang, Yuan Qing, and Eric Jacobsen. “Cooperative, Highly Enantioselective Phosphinothiourea Catalysis of Imine−Allene [3 + 2] Cycloadditions.” Journal of the American Chemical Society, vol. 130, no. 17, Apr. 2008, pp. 5660-5661. https://doi.org/10.1021/ja801344w.
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