Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes
Svetlana Kyatskaya
1
,
José Ramón Galán-Mascarós
1
,
L. Bogani
1
,
Frank Hennrich
1
,
Manfred M. Kappes
1
,
Mario Ruben
1
Publication type: Journal Article
Publication date: 2009-10-02
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
19799421
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
A new heteroleptic bis(phthalocyaninato) terbium(III) complex 1, bearing a pyrenyl group, exhibits temperature and frequency dependence of ac magnetic susceptibility, typical of single-molecule magnets. The complex was successfully attached to single-walled carbon nanotubes (SWNTs) using pi-pi interactions, yielding a 1-SWNT conjugate. The supramolecular grafting of 1 to SWNTs was proven qualitatively and quantitatively by high-resolution transmission electron microscopy, emission spectroscopy, and atomic force spectroscopy. Giving a clear magnetic fingerprint, the anisotropy energy barrier and the magnetic relaxation time of the 1-SWNT conjugate are both increased in comparison with the pure crystalline compound 1, likely due to the suppression of intermolecular interactions. The obtained results propose the 1-SWNT conjugate as a promising constituent unit in magnetic single-molecule measurements using molecular spintronics devices.
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187
Total citations:
187
Citations from 2025:
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(3.74%)
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GOST
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Kyatskaya S. et al. Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes // Journal of the American Chemical Society. 2009. Vol. 131. No. 42. pp. 15143-15151.
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Kyatskaya S., Galán-Mascarós J. R., Bogani L., Hennrich F., Kappes M. M., Wernsdorfer W., Ruben M. Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes // Journal of the American Chemical Society. 2009. Vol. 131. No. 42. pp. 15143-15151.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ja906165e
UR - https://doi.org/10.1021/ja906165e
TI - Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes
T2 - Journal of the American Chemical Society
AU - Kyatskaya, Svetlana
AU - Galán-Mascarós, José Ramón
AU - Bogani, L.
AU - Hennrich, Frank
AU - Kappes, Manfred M.
AU - Wernsdorfer, Wolfgang
AU - Ruben, Mario
PY - 2009
DA - 2009/10/02
PB - American Chemical Society (ACS)
SP - 15143-15151
IS - 42
VL - 131
PMID - 19799421
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
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@article{2009_Kyatskaya,
author = {Svetlana Kyatskaya and José Ramón Galán-Mascarós and L. Bogani and Frank Hennrich and Manfred M. Kappes and Wolfgang Wernsdorfer and Mario Ruben},
title = {Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes},
journal = {Journal of the American Chemical Society},
year = {2009},
volume = {131},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/ja906165e},
number = {42},
pages = {15143--15151},
doi = {10.1021/ja906165e}
}
Cite this
MLA
Copy
Kyatskaya, Svetlana, et al. “Anchoring of Rare-Earth-Based Single-Molecule Magnets on Single-Walled Carbon Nanotubes.” Journal of the American Chemical Society, vol. 131, no. 42, Oct. 2009, pp. 15143-15151. https://doi.org/10.1021/ja906165e.