Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins.
Publication type: Journal Article
Publication date: 2009-11-24
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
19929002
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
A new strategy for gold and palladium dual-catalytic reactivity and turnover, called catalyzed catalysis, enhanced the synthetic usefulness of vinylgold intermediates by providing dual-catalytic carbon-carbon cross-coupling as an alternative to protodemetalation. This protocol enabled the synthesis of substituted butenolides and isocoumarins from allyl esters. Kinetic and spectroscopic experiments support a mechanism in which the Lewis acidic gold complex catalyzes both an initial rearrangement step and a subsequent Lewis basic palladium oxidative-addition step.
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228
Total citations:
228
Citations from 2024:
8
(3.51%)
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GOST
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Shi Y. et al. Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins. // Journal of the American Chemical Society. 2009. Vol. 131. No. 50. pp. 18022-18023.
GOST all authors (up to 50)
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Shi Y., Roth K. E., Ramgren S. D., Blum S. A. Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins. // Journal of the American Chemical Society. 2009. Vol. 131. No. 50. pp. 18022-18023.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ja9068497
UR - https://doi.org/10.1021/ja9068497
TI - Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins.
T2 - Journal of the American Chemical Society
AU - Shi, Yili
AU - Roth, Katrina E
AU - Ramgren, Stephen D
AU - Blum, Suzanne A
PY - 2009
DA - 2009/11/24
PB - American Chemical Society (ACS)
SP - 18022-18023
IS - 50
VL - 131
PMID - 19929002
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2009_Shi,
author = {Yili Shi and Katrina E Roth and Stephen D Ramgren and Suzanne A Blum},
title = {Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins.},
journal = {Journal of the American Chemical Society},
year = {2009},
volume = {131},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/ja9068497},
number = {50},
pages = {18022--18023},
doi = {10.1021/ja9068497}
}
Cite this
MLA
Copy
Shi, Yili, et al. “Catalyzed catalysis using carbophilic Lewis acidic gold and Lewis basic palladium: synthesis of substituted butenolides and isocoumarins..” Journal of the American Chemical Society, vol. 131, no. 50, Nov. 2009, pp. 18022-18023. https://doi.org/10.1021/ja9068497.