Journal of the American Chemical Society, volume 131, issue 50, pages 18036-18037

Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state.

Shao-Liang Zheng ¹

Yizhong Wang ¹

Zhipeng Yu ¹

Qing Lin ¹

Philip Coppens ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Department of Chemistry, State University of New York at Buffalo, Buffalo, New York 14260 |

Publication type: Journal Article

Publication date: 2009-11-24

American Chemical Society (ACS)

Journal: Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor: 15

ISSN: 00027863, 15205126

DOI: 10.1021/ja9094523

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PubMed ID: 19928921

General Chemistry

Catalysis

Biochemistry

Colloid and Surface Chemistry

Abstract

We report the direct observation of a bent geometry for a nonstabilized nitrile imine in a metal-coordination crystal. The photoinduced tetrazole ring rupture to release N(2) appears to depend on the size of voids around the N(3)-N(4) bond in the crystal lattice. We further observed the selective formation of the 1,3-addition product when a reactive nitrile imine was photogenerated in water. Overall, the bent nitrile imine geometry agrees with the 1,3-dipolar structure, a transient reactive species that mediates the photoinduced 1,3-dipolar cycloaddition in the aqueous medium.

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Citations by journals

	1 2 3 4 5 6
Journal of the American Chemical Society	Journal of the American Chemical Society, 6, 10.17% Journal of the American Chemical Society 6 publications, 10.17%
Chemical Communications	Chemical Communications, 6, 10.17% Chemical Communications 6 publications, 10.17%
Angewandte Chemie	Angewandte Chemie, 3, 5.08% Angewandte Chemie 3 publications, 5.08%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 3, 5.08% Angewandte Chemie - International Edition 3 publications, 5.08%
Advanced Functional Materials	Advanced Functional Materials, 3, 5.08% Advanced Functional Materials 3 publications, 5.08%
Topics in Current Chemistry	Topics in Current Chemistry, 2, 3.39% Topics in Current Chemistry 2 publications, 3.39%
Russian Chemical Reviews	Russian Chemical Reviews, 2, 3.39% Russian Chemical Reviews 2 publications, 3.39%
Crystal Growth and Design	Crystal Growth and Design, 2, 3.39% Crystal Growth and Design 2 publications, 3.39%
Inorganic Chemistry	Inorganic Chemistry, 2, 3.39% Inorganic Chemistry 2 publications, 3.39%
Chemical Science	Chemical Science, 2, 3.39% Chemical Science 2 publications, 3.39%
Bioconjugate Chemistry	Bioconjugate Chemistry, 1, 1.69% Bioconjugate Chemistry 1 publication, 1.69%
Chemistry Letters	Chemistry Letters, 1, 1.69% Chemistry Letters 1 publication, 1.69%
IUCrData	IUCrData, 1, 1.69% IUCrData 1 publication, 1.69%
Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials	Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials, 1, 1.69% Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials 1 publication, 1.69%
Acta Crystallographica Section E: Crystallographic Communications	Acta Crystallographica Section E: Crystallographic Communications, 1, 1.69% Acta Crystallographica Section E: Crystallographic Communications 1 publication, 1.69%
Molecules	Molecules, 1, 1.69% Molecules 1 publication, 1.69%
Crystals	Crystals, 1, 1.69% Crystals 1 publication, 1.69%
Photochemical and Photobiological Sciences	Photochemical and Photobiological Sciences, 1, 1.69% Photochemical and Photobiological Sciences 1 publication, 1.69%
Science China Chemistry	Science China Chemistry, 1, 1.69% Science China Chemistry 1 publication, 1.69%
Chemical Research in Chinese Universities	Chemical Research in Chinese Universities, 1, 1.69% Chemical Research in Chinese Universities 1 publication, 1.69%
European Polymer Journal	European Polymer Journal, 1, 1.69% European Polymer Journal 1 publication, 1.69%
Renewable and Sustainable Energy Reviews	Renewable and Sustainable Energy Reviews, 1, 1.69% Renewable and Sustainable Energy Reviews 1 publication, 1.69%
Inorganic Chemistry Communication	Inorganic Chemistry Communication, 1, 1.69% Inorganic Chemistry Communication 1 publication, 1.69%
Progress in Polymer Science	Progress in Polymer Science, 1, 1.69% Progress in Polymer Science 1 publication, 1.69%
Dyes and Pigments	Dyes and Pigments, 1, 1.69% Dyes and Pigments 1 publication, 1.69%
European Journal of Inorganic Chemistry	European Journal of Inorganic Chemistry, 1, 1.69% European Journal of Inorganic Chemistry 1 publication, 1.69%
ChemBioChem	ChemBioChem, 1, 1.69% ChemBioChem 1 publication, 1.69%
Chemistry - A European Journal	Chemistry - A European Journal, 1, 1.69% Chemistry - A European Journal 1 publication, 1.69%
European Journal of Organic Chemistry	European Journal of Organic Chemistry, 1, 1.69% European Journal of Organic Chemistry 1 publication, 1.69%
Accounts of Chemical Research	Accounts of Chemical Research, 1, 1.69% Accounts of Chemical Research 1 publication, 1.69%
	1 2 3 4 5 6

Citations by publishers

	2 4 6 8 10 12 14 16
American Chemical Society (ACS)	American Chemical Society (ACS), 15, 25.42% American Chemical Society (ACS) 15 publications, 25.42%
Wiley	Wiley, 13, 22.03% Wiley 13 publications, 22.03%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 9, 15.25% Royal Society of Chemistry (RSC) 9 publications, 15.25%
Elsevier	Elsevier, 7, 11.86% Elsevier 7 publications, 11.86%
Springer Nature	Springer Nature, 5, 8.47% Springer Nature 5 publications, 8.47%
International Union of Crystallography (IUCr)	International Union of Crystallography (IUCr), 3, 5.08% International Union of Crystallography (IUCr) 3 publications, 5.08%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 3.39% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 3.39%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 3.39% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 3.39%
The Chemical Society of Japan	The Chemical Society of Japan, 1, 1.69% The Chemical Society of Japan 1 publication, 1.69%
Taylor & Francis	Taylor & Francis, 1, 1.69% Taylor & Francis 1 publication, 1.69%
	2 4 6 8 10 12 14 16

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Zheng S. et al. Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state. // Journal of the American Chemical Society. 2009. Vol. 131. No. 50. pp. 18036-18037.

GOST all authors (up to 50) Copy

Zheng S., Wang Y., Yu Z., Lin Q., Coppens P. Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state. // Journal of the American Chemical Society. 2009. Vol. 131. No. 50. pp. 18036-18037.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/ja9094523

UR - https://doi.org/10.1021/ja9094523

TI - Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state.

T2 - Journal of the American Chemical Society

AU - Wang, Yizhong

AU - Coppens, Philip

AU - Zheng, Shao-Liang

AU - Yu, Zhipeng

AU - Lin, Qing

PY - 2009

DA - 2009/11/24 00:00:00

PB - American Chemical Society (ACS)

SP - 18036-18037

IS - 50

VL - 131

PMID - 19928921

SN - 0002-7863

SN - 1520-5126

ER -

BibTex |

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BibTex Copy

@article{2009_Zheng,

author = {Yizhong Wang and Philip Coppens and Shao-Liang Zheng and Zhipeng Yu and Qing Lin},

title = {Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state.},

journal = {Journal of the American Chemical Society},

year = {2009},

volume = {131},

publisher = {American Chemical Society (ACS)},

month = {nov},

url = {https://doi.org/10.1021/ja9094523},

number = {50},

pages = {18036--18037},

doi = {10.1021/ja9094523}

}

MLA

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MLA Copy

Zheng, Shao-Liang, et al. “Direct observation of a photoinduced nonstabilized nitrile imine structure in the solid state..” Journal of the American Chemical Society, vol. 131, no. 50, Nov. 2009, pp. 18036-18037. https://doi.org/10.1021/ja9094523.

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Publisher

American Chemical Society (ACS)

Journal

Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

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00027863 (Print)
15205126 (Electronic)