Journal of the American Chemical Society, volume 142, issue 15, pages 7012-7022

Site-Occupation-Tuned Superionic Li_xScCl_3+xHalide Solid Electrolytes for All-Solid-State Batteries

Jianwen Liang ¹

Xiaona Li ¹

Shuo Wang ²

Keegan Adair ¹

Weihan Li ¹

Yang Zhao ¹

Changhong Wang ¹

Yongfeng Hu ³

Li Zhang ⁴

Shangqian Zhao ⁴

Shigang Lu ⁴

Huan Huang ⁵

Ruying Li ¹

Yifei Mo ²

Xueliang Andy Sun ¹

Hide authors affiliations Show authors affiliations: 5 affiliations

Department of Mechanical and Materials Engineering, University of Western Ontario, 1151 Richmond St, London, Ontario N6A 3K7, Canada |

Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, United States |

Canadian Light Source, 44 Innovation Boulevard, Saskatoon, SK S7N 2V3, Canada |

⁴

China Automotive Battery Research Institute Co. Ltd, fifth Floor, No. 43, Mining Building, North Sanhuan Middle Road, Beijing, 100088, China |

⁵

Glabat Solid-State Battery Inc., 700 Collip Circle, London, ON N6G 4X8, Canada |

Publication type: Journal Article

Publication date: 2020-03-26

American Chemical Society (ACS)

Journal: Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor: 15

ISSN: 00027863, 15205126

DOI: 10.1021/jacs.0c00134

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General Chemistry

Catalysis

Biochemistry

Colloid and Surface Chemistry

Abstract

The enabling of high energy density of all-solid-state lithium batteries (ASSLBs) requires the development of highly Li+-conductive solid-state electrolytes (SSEs) with good chemical and electrochemical stability. Recently, halide SSEs based on different material design principles have opened new opportunities for ASSLBs. Here, we discovered a series of LixScCl3+x SSEs (x = 2.5, 3, 3.5, and 4) based on the cubic close-packed anion sublattice with room-temperature ionic conductivities up to 3 × 10-3 S cm-1. Owing to the low eutectic temperature between LiCl and ScCl3, LixScCl3+x SSEs can be synthesized by a simple co-melting strategy. Preferred orientation is observed for all the samples. The influence of the value of x in LixScCl3+x on the structure and Li+ diffusivity were systematically explored. With increasing x value, higher Li+, lower vacancy concentration, and less blocking effects from Sc ions are achieved, enabling the ability to tune the Li+ migration. The electrochemical performance shows that Li3ScCl6 possesses a wide electrochemical window of 0.9-4.3 V vs Li+/Li, stable electrochemical plating/stripping of Li for over 2500 h, as well as good compatibility with LiCoO2. LiCoO2/Li3ScCl6/In ASSLB exhibits a reversible capacity of 104.5 mAh g-1 with good cycle life retention for 160 cycles. The observed changes in the ionic conductivity and tuning of the site occupations provide an additional approach toward the design of better SSEs.

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Citations by journals

	2 4 6 8 10 12 14 16 18
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 18, 5.92% Journal of Materials Chemistry A 18 publications, 5.92%
ACS applied materials & interfaces	ACS applied materials & interfaces, 18, 5.92% ACS applied materials & interfaces 18 publications, 5.92%
Advanced Energy Materials	Advanced Energy Materials, 18, 5.92% Advanced Energy Materials 18 publications, 5.92%
ACS Energy Letters	ACS Energy Letters, 15, 4.93% ACS Energy Letters 15 publications, 4.93%
Energy Storage Materials	Energy Storage Materials, 13, 4.28% Energy Storage Materials 13 publications, 4.28%
Nature Communications	Nature Communications, 10, 3.29% Nature Communications 10 publications, 3.29%
Journal of the American Chemical Society	Journal of the American Chemical Society, 9, 2.96% Journal of the American Chemical Society 9 publications, 2.96%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 9, 2.96% Angewandte Chemie - International Edition 9 publications, 2.96%
Chemistry of Materials	Chemistry of Materials, 9, 2.96% Chemistry of Materials 9 publications, 2.96%
Advanced Materials	Advanced Materials, 9, 2.96% Advanced Materials 9 publications, 2.96%
Angewandte Chemie	Angewandte Chemie, 9, 2.96% Angewandte Chemie 9 publications, 2.96%
Journal of Power Sources	Journal of Power Sources, 8, 2.63% Journal of Power Sources 8 publications, 2.63%
ACS Applied Energy Materials	ACS Applied Energy Materials, 7, 2.3% ACS Applied Energy Materials 7 publications, 2.3%
Chemical Engineering Journal	Chemical Engineering Journal, 7, 2.3% Chemical Engineering Journal 7 publications, 2.3%
Advanced Functional Materials	Advanced Functional Materials, 6, 1.97% Advanced Functional Materials 6 publications, 1.97%
Advanced Science	Advanced Science, 6, 1.97% Advanced Science 6 publications, 1.97%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 5, 1.64% Journal of Physical Chemistry C 5 publications, 1.64%
Energy and Environmental Science	Energy and Environmental Science, 5, 1.64% Energy and Environmental Science 5 publications, 1.64%
Nano Energy	Nano Energy, 4, 1.32% Nano Energy 4 publications, 1.32%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 4, 1.32% Electrochemical Energy Reviews 4 publications, 1.32%
Nano Letters	Nano Letters, 4, 1.32% Nano Letters 4 publications, 1.32%
Chemical Science	Chemical Science, 4, 1.32% Chemical Science 4 publications, 1.32%
Science advances	Science advances, 4, 1.32% Science advances 4 publications, 1.32%
ACS Materials Letters	ACS Materials Letters, 3, 0.99% ACS Materials Letters 3 publications, 0.99%
Nano Research	Nano Research, 3, 0.99% Nano Research 3 publications, 0.99%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 3, 0.99% Journal of Solid State Electrochemistry 3 publications, 0.99%
Joule	Joule, 3, 0.99% Joule 3 publications, 0.99%
Chinese Chemical Letters	Chinese Chemical Letters, 3, 0.99% Chinese Chemical Letters 3 publications, 0.99%
Small	Small, 3, 0.99% Small 3 publications, 0.99%
	2 4 6 8 10 12 14 16 18

Citations by publishers

	10 20 30 40 50 60 70 80
American Chemical Society (ACS)	American Chemical Society (ACS), 78, 25.66% American Chemical Society (ACS) 78 publications, 25.66%
Wiley	Wiley, 70, 23.03% Wiley 70 publications, 23.03%
Elsevier	Elsevier, 67, 22.04% Elsevier 67 publications, 22.04%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 34, 11.18% Royal Society of Chemistry (RSC) 34 publications, 11.18%
Springer Nature	Springer Nature, 33, 10.86% Springer Nature 33 publications, 10.86%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 4, 1.32% American Association for the Advancement of Science (AAAS) 4 publications, 1.32%
The Electrochemical Society	The Electrochemical Society, 3, 0.99% The Electrochemical Society 3 publications, 0.99%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 0.66% American Institute of Physics (AIP) 2 publications, 0.66%
IOP Publishing	IOP Publishing, 2, 0.66% IOP Publishing 2 publications, 0.66%
Chinese Physical Society	Chinese Physical Society, 2, 0.66% Chinese Physical Society 2 publications, 0.66%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 2, 0.66% The Electrochemical Society of Japan 2 publications, 0.66%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.33% Frontiers Media S.A. 1 publication, 0.33%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.33% Nonferrous Metals Society of China 1 publication, 0.33%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.33% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.33%
The Chemical Society of Japan	The Chemical Society of Japan, 1, 0.33% The Chemical Society of Japan 1 publication, 0.33%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.33% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.33%
	10 20 30 40 50 60 70 80

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Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
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Liang J. et al. Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries // Journal of the American Chemical Society. 2020. Vol. 142. No. 15. pp. 7012-7022.

GOST all authors (up to 50) Copy

Liang J., Li X., Wang S., Adair K., Li W., Zhao Y., Wang C., Hu Y., Zhang L., Zhao S., Lu S., Huang H., Li R., Mo Y., Sun X. A. Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries // Journal of the American Chemical Society. 2020. Vol. 142. No. 15. pp. 7012-7022.

RIS |

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TY - JOUR

DO - 10.1021/jacs.0c00134

UR - https://doi.org/10.1021/jacs.0c00134

TI - Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries

T2 - Journal of the American Chemical Society

AU - Li, Weihan

AU - Zhao, Shangqian

AU - Lu, Shigang

AU - Wang, Shuo

AU - Mo, Yifei

AU - Sun, Xueliang Andy

AU - Liang, Jianwen

AU - Li, Xiaona

AU - Adair, Keegan

AU - Zhao, Yang

AU - Wang, Changhong

AU - Hu, Yongfeng

AU - Zhang, Li

AU - Huang, Huan

AU - Li, Ruying

PY - 2020

DA - 2020/03/26 00:00:00

PB - American Chemical Society (ACS)

SP - 7012-7022

IS - 15

VL - 142

SN - 0002-7863

SN - 1520-5126

ER -

BibTex |

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BibTex Copy

@article{2020_Liang,

author = {Weihan Li and Shangqian Zhao and Shigang Lu and Shuo Wang and Yifei Mo and Xueliang Andy Sun and Jianwen Liang and Xiaona Li and Keegan Adair and Yang Zhao and Changhong Wang and Yongfeng Hu and Li Zhang and Huan Huang and Ruying Li},

title = {Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries},

journal = {Journal of the American Chemical Society},

year = {2020},

volume = {142},

publisher = {American Chemical Society (ACS)},

month = {mar},

url = {https://doi.org/10.1021/jacs.0c00134},

number = {15},

pages = {7012--7022},

doi = {10.1021/jacs.0c00134}

}

MLA

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MLA Copy

Liang, Jianwen, et al. “Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries.” Journal of the American Chemical Society, vol. 142, no. 15, Mar. 2020, pp. 7012-7022. https://doi.org/10.1021/jacs.0c00134.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor

ISSN

00027863 (Print)
15205126 (Electronic)