Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones
Тип публикации: Journal Article
Дата публикации: 2021-02-09
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 5.491
CiteScore: 22
Impact factor: 16.6
ISSN: 00027863, 15205126
PubMed ID:
33560837
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Краткое описание
A palladium-catalyzed imidoylative cycloamidation of N-alkyl-2-isocyanobenzamides with 2,6-disubstituted aryl iodides, affording unprecedented axially chiral 2-arylquinazolinones, has been developed with good yields and atroposelectivities. In this coupling-cyclization process, the biaryl linkage and the heteroaromatic ring are formed sequentially in one step. When N-(2,4-dimethoxyphenyl)-2-isocyanobenzamide is applied as a substrate, 2,3-diarylquinazolinones containing two stereogenic axes are produced with moderate diastereoselectivity and good enantioselectivities.
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Fan T. et al. Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones // Journal of the American Chemical Society. 2021. Vol. 143. No. 7. pp. 2722-2728.
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Fan T., Yu Ting T., Peng Y., Hu W., Hu H., He Y., Luo S., Zhu Q. Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones // Journal of the American Chemical Society. 2021. Vol. 143. No. 7. pp. 2722-2728.
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TY - JOUR
DO - 10.1021/jacs.1c00640
UR - https://doi.org/10.1021/jacs.1c00640
TI - Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones
T2 - Journal of the American Chemical Society
AU - Fan, Teng
AU - Yu Ting, Ting
AU - Peng, Yan
AU - Hu, Weiming
AU - Hu, Huaanzi
AU - He, Yimiao
AU - Luo, Shuang
AU - Zhu, Qiang
PY - 2021
DA - 2021/02/09
PB - American Chemical Society (ACS)
SP - 2722-2728
IS - 7
VL - 143
PMID - 33560837
SN - 0002-7863
SN - 1520-5126
ER -
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BibTex (до 50 авторов)
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@article{2021_Fan,
author = {Teng Fan and Ting Yu Ting and Yan Peng and Weiming Hu and Huaanzi Hu and Yimiao He and Shuang Luo and Qiang Zhu},
title = {Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones},
journal = {Journal of the American Chemical Society},
year = {2021},
volume = {143},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/jacs.1c00640},
number = {7},
pages = {2722--2728},
doi = {10.1021/jacs.1c00640}
}
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MLA
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Fan, Teng, et al. “Palladium-Catalyzed Atroposelective Coupling–Cyclization of 2-Isocyanobenzamides to Construct Axially Chiral 2-Aryl- and 2,3-Diarylquinazolinones.” Journal of the American Chemical Society, vol. 143, no. 7, Feb. 2021, pp. 2722-2728. https://doi.org/10.1021/jacs.1c00640.
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